Density modes in spherical 4He shells

We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional des...

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Autores principales: Barranco, M., Hernández, E.S., Mayol, R., Pi, M.
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Acceso en línea:http://hdl.handle.net/20.500.12110/paper_01631829_v69_n13_p134502_Barranco
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spelling todo:paper_01631829_v69_n13_p134502_Barranco2023-10-03T15:01:56Z Density modes in spherical 4He shells Barranco, M. Hernández, E.S. Mayol, R. Pi, M. carbon fullerene helium article chemical structure density density functional theory elementary particle excitation geometry hydrodynamics mathematical analysis quantum mechanics We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional description of the shell structure. The presence of one or two solid helium layers adjacent to the adsorbing fullerene is phenomenologically accounted for. We illustrate our results for a selection of numbers of adsorbed atoms on C20, C 60, and C120. The hydrodynamical model that has proven successful to describe helium excitations in the bulk and in restricted geometries permits to perform a rather exhaustive analysis of various fluid spherical systems, namely, spheres, cavities, free bubbles, and bound shells of variable size. Fil:Hernández, E.S. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales; Argentina. JOUR info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/2.5/ar http://hdl.handle.net/20.500.12110/paper_01631829_v69_n13_p134502_Barranco
institution Universidad de Buenos Aires
institution_str I-28
repository_str R-134
collection Biblioteca Digital - Facultad de Ciencias Exactas y Naturales (UBA)
topic carbon
fullerene
helium
article
chemical structure
density
density functional theory
elementary particle
excitation
geometry
hydrodynamics
mathematical analysis
quantum mechanics
spellingShingle carbon
fullerene
helium
article
chemical structure
density
density functional theory
elementary particle
excitation
geometry
hydrodynamics
mathematical analysis
quantum mechanics
Barranco, M.
Hernández, E.S.
Mayol, R.
Pi, M.
Density modes in spherical 4He shells
topic_facet carbon
fullerene
helium
article
chemical structure
density
density functional theory
elementary particle
excitation
geometry
hydrodynamics
mathematical analysis
quantum mechanics
description We compute the density-fluctuation spectrum of spherical 4HeN shells adsorbed on the outer surface of C n fullerenes. The excitation spectrum is obtained within the random-phase approximation, with particle-hole elementary excitations and effective interaction extracted from a density-functional description of the shell structure. The presence of one or two solid helium layers adjacent to the adsorbing fullerene is phenomenologically accounted for. We illustrate our results for a selection of numbers of adsorbed atoms on C20, C 60, and C120. The hydrodynamical model that has proven successful to describe helium excitations in the bulk and in restricted geometries permits to perform a rather exhaustive analysis of various fluid spherical systems, namely, spheres, cavities, free bubbles, and bound shells of variable size.
format JOUR
author Barranco, M.
Hernández, E.S.
Mayol, R.
Pi, M.
author_facet Barranco, M.
Hernández, E.S.
Mayol, R.
Pi, M.
author_sort Barranco, M.
title Density modes in spherical 4He shells
title_short Density modes in spherical 4He shells
title_full Density modes in spherical 4He shells
title_fullStr Density modes in spherical 4He shells
title_full_unstemmed Density modes in spherical 4He shells
title_sort density modes in spherical 4he shells
url http://hdl.handle.net/20.500.12110/paper_01631829_v69_n13_p134502_Barranco
work_keys_str_mv AT barrancom densitymodesinspherical4heshells
AT hernandezes densitymodesinspherical4heshells
AT mayolr densitymodesinspherical4heshells
AT pim densitymodesinspherical4heshells
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