A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril

Di–hydroxymethyl–di–2–(pyrrolyl)methane (DMPM) and 7,7,8,8–tetracyanoquinodimethane (TCNQ) were dissolved in acetonitrile to form a π–π charge–transfer complex, which exhibits a deep blue color. This complex is decomposed with the addition of captopril. It was possible to observe a change from the v...

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Autores principales: Torri, Eliane, Nicoleti, Celso R., Zimmermann, Lizandra M., Machado, Vanderlei G.
Formato: Articulo
Lenguaje:Inglés
Publicado: 2012
Materias:
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/20222
http://www.latamjpharm.org/resumenes/31/5/LAJOP_31_5_1_10.pdf
Aporte de:
id I19-R120-10915-20222
record_format dspace
institution Universidad Nacional de La Plata
institution_str I-19
repository_str R-120
collection SEDICI (UNLP)
language Inglés
topic Farmacia
Captopril
Chromogenic chemosensors
Displacement assay
Naked-eye detection
TCNQ
Metano
spellingShingle Farmacia
Captopril
Chromogenic chemosensors
Displacement assay
Naked-eye detection
TCNQ
Metano
Torri, Eliane
Nicoleti, Celso R.
Zimmermann, Lizandra M.
Machado, Vanderlei G.
A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
topic_facet Farmacia
Captopril
Chromogenic chemosensors
Displacement assay
Naked-eye detection
TCNQ
Metano
description Di–hydroxymethyl–di–2–(pyrrolyl)methane (DMPM) and 7,7,8,8–tetracyanoquinodimethane (TCNQ) were dissolved in acetonitrile to form a π–π charge–transfer complex, which exhibits a deep blue color. This complex is decomposed with the addition of captopril. It was possible to observe a change from the vivid blue color to pale orange–yellow, which is related to the formation of a new n–π complex between TCNQ and captopril. The formation kinetics of the complex between DMPM and TCNQ in acetonitrile was studied, it being concluded that the interaction between the two compounds is a photochemical process. Spectrophotometric titrations of TCNQ with DMPM were carried out and the results demonstrated that, in acetonitrile, the complex formed comprises one molecule of TCNQ for two of DMPM while in an acetonitrile:water mixture (9:1; v/v) a change to a 1:1 stoichiometry was observed.
format Articulo
Articulo
author Torri, Eliane
Nicoleti, Celso R.
Zimmermann, Lizandra M.
Machado, Vanderlei G.
author_facet Torri, Eliane
Nicoleti, Celso R.
Zimmermann, Lizandra M.
Machado, Vanderlei G.
author_sort Torri, Eliane
title A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
title_short A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
title_full A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
title_fullStr A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
title_full_unstemmed A chromogenic chemosensor based on a complex of Di–Hydroxymethyl–Di–2–(Pyrrolyl)Methane and 7,7,8,8–Tetracyanoquinodimethane for the detection of captopril
title_sort chromogenic chemosensor based on a complex of di–hydroxymethyl–di–2–(pyrrolyl)methane and 7,7,8,8–tetracyanoquinodimethane for the detection of captopril
publishDate 2012
url http://sedici.unlp.edu.ar/handle/10915/20222
http://www.latamjpharm.org/resumenes/31/5/LAJOP_31_5_1_10.pdf
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