S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group

There is a major need for light-activated materials for the release of sensitizers and drugs. Considering the success of chiral columns for the separation of enantiomer drugs, we synthesized an S,S-chiral linker system covalently attached to silica with a sensitizer ethene near the silica surface....

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Autores principales: Ghosh, Goutam, Belh, Sarah J., Chiemezie, Callistus, Walalawela, Niluksha, Ghogare, Ashwini A., Vignoni, Mariana, Thomas, Andrés Héctor, McFarland, Sherri A., Greer, Edyta M., Greer, Alexander
Formato: Articulo Preprint
Lenguaje:Inglés
Publicado: 2019
Materias:
Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/107002
http://europepmc.org/backend/ptpmcrender.fcgi?accid=PMC6347524&blobtype=pdf
Aporte de:
id I19-R120-10915-107002
record_format dspace
institution Universidad Nacional de La Plata
institution_str I-19
repository_str R-120
collection SEDICI (UNLP)
language Inglés
topic Química
S,S-chiral linker system
Drug photorelease
spellingShingle Química
S,S-chiral linker system
Drug photorelease
Ghosh, Goutam
Belh, Sarah J.
Chiemezie, Callistus
Walalawela, Niluksha
Ghogare, Ashwini A.
Vignoni, Mariana
Thomas, Andrés Héctor
McFarland, Sherri A.
Greer, Edyta M.
Greer, Alexander
S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
topic_facet Química
S,S-chiral linker system
Drug photorelease
description There is a major need for light-activated materials for the release of sensitizers and drugs. Considering the success of chiral columns for the separation of enantiomer drugs, we synthesized an S,S-chiral linker system covalently attached to silica with a sensitizer ethene near the silica surface. First, the silica surface was modified to be aromatic rich, by replacing 70% of the surface groups with (3-phenoxypropyl)silane. We then synthesized a 3-component conjugate [chlorin sensitizer, S,S-chiral cyclohexane, and ethene building blocks] in 5 steps with a 13% yield, and covalently bound the conjugate to the (3-phenoxypropyl)silane-coated silica surface. We hypothesized that the chiral linker would increase exposure of the ethene site for enhanced 1O2- based sensitizer release. However, the chiral linker caused the sensitizer conjugate to adopt a Ushape due to favored 1,2-diaxial substituent orientation; resulting in a reduced efficiency of surface loading. Further accentuating the U-shape was π–π stacking between the (3-phenoxypropyl)silane and sensitizer. Semiempirical calculations and singlet oxygen luminescence data provided deeper insight into the sensitizer’s orientation and release. This study has lead to insight on modifications of surfaces for drug photorelease and can help lead to the development of miniaturized photodynamic devices.
format Articulo
Preprint
author Ghosh, Goutam
Belh, Sarah J.
Chiemezie, Callistus
Walalawela, Niluksha
Ghogare, Ashwini A.
Vignoni, Mariana
Thomas, Andrés Héctor
McFarland, Sherri A.
Greer, Edyta M.
Greer, Alexander
author_facet Ghosh, Goutam
Belh, Sarah J.
Chiemezie, Callistus
Walalawela, Niluksha
Ghogare, Ashwini A.
Vignoni, Mariana
Thomas, Andrés Héctor
McFarland, Sherri A.
Greer, Edyta M.
Greer, Alexander
author_sort Ghosh, Goutam
title S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
title_short S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
title_full S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
title_fullStr S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
title_full_unstemmed S,S-Chiral Linker Induced U Shape with a Syn-facial Sensitizer and Photocleavable Ethene Group
title_sort s,s-chiral linker induced u shape with a syn-facial sensitizer and photocleavable ethene group
publishDate 2019
url http://sedici.unlp.edu.ar/handle/10915/107002
http://europepmc.org/backend/ptpmcrender.fcgi?accid=PMC6347524&blobtype=pdf
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