Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments

A green method is reported based on non-sophisticated instrumental for the quantification of seven natural and synthetic estrogens, three progestagens and one androgen in the presence of real interferences. The method takes advantage of: (1) chromatography, allowing total or partial resolution of a...

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Autores principales: Pérez, Rocío Laura, Escandar, Graciela Mónica
Lenguaje:Inglés
Publicado: Elsevier 2018
Materias:
Acceso en línea:http://hdl.handle.net/2133/11454
http://hdl.handle.net/2133/11454
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id I15-R121-2133-11454
record_format dspace
institution Universidad Nacional de Rosario
institution_str I-15
repository_str R-121
collection Repositorio Hipermedial de la Universidad Nacional de Rosario (UNR)
language Inglés
orig_language_str_mv eng
topic High-performance-liquid Chromatography
Dual UV-fluorescence Detection
Multivariate Curve Resolution
Endocrine Disruptors
Environmental Samples
spellingShingle High-performance-liquid Chromatography
Dual UV-fluorescence Detection
Multivariate Curve Resolution
Endocrine Disruptors
Environmental Samples
Pérez, Rocío Laura
Escandar, Graciela Mónica
Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
topic_facet High-performance-liquid Chromatography
Dual UV-fluorescence Detection
Multivariate Curve Resolution
Endocrine Disruptors
Environmental Samples
description A green method is reported based on non-sophisticated instrumental for the quantification of seven natural and synthetic estrogens, three progestagens and one androgen in the presence of real interferences. The method takes advantage of: (1) chromatography, allowing total or partial resolution of a large number of compounds, (2) dual detection, permitting selection of the most appropriate signal for each analyte and, (3) second-order calibration, enabling mathematical resolution of incompletely resolved chromatographic bands and analyte determination in the presence of interferents. Consumption of organic solvents for cleaning, extraction and separation are markedly decreased because of the coupling with MCR-ALS (multivariate curve resolution/alternating least-squares) which allows the successful resolution in the presence of other co-eluting matrix constituents. Rigorous IUPAC detection limits were obtained: 6–24 ng L−1 in water, and 0.1–0.9 ng g−1 in sediments. Relative prediction errors were 2–10% (water) and 1–8% (sediments).
author Pérez, Rocío Laura
Escandar, Graciela Mónica
author_facet Pérez, Rocío Laura
Escandar, Graciela Mónica
author_sort Pérez, Rocío Laura
title Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
title_short Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
title_full Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
title_fullStr Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
title_full_unstemmed Multivariate calibration-assisted high-performance liquid chromatography with dual UV and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
title_sort multivariate calibration-assisted high-performance liquid chromatography with dual uv and fluorimetric detection for the analysis of natural and synthetic sex hormones in environmental waters and sediments
publisher Elsevier
publishDate 2018
url http://hdl.handle.net/2133/11454
http://hdl.handle.net/2133/11454
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AT escandargracielamonica multivariatecalibrationassistedhighperformanceliquidchromatographywithdualuvandfluorimetricdetectionfortheanalysisofnaturalandsyntheticsexhormonesinenvironmentalwatersandsediments
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