Screening of one-bead-one-peptide combinatorial library using red fluorescent dyes. Presence of positive and false positive beads

To screen one-bead-one-compound (OBOC) combinatorial libraries, tens of thousands to millions of compound beads are first mixed with a target molecule. The beads that interact with this molecule are then identified and isolated for compound structure determination. Here we describe an OBOC peptide l...

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Autor principal: Marani, M.M
Otros Autores: Ceron, M.C.M, Giudicessi, S.L, De Oliveira, E., Côté, S., Erra-Balsells, R., Albericio, F., Cascone, O., Camperi, S.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2009
Acceso en línea:Registro en Scopus
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Registro en la Biblioteca Digital
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024 7 |2 scopus  |a 2-s2.0-60849100790 
024 7 |2 cas  |a Fluorescent Dyes; Peptide Library 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a JCCHF 
100 1 |a Marani, M.M. 
245 1 0 |a Screening of one-bead-one-peptide combinatorial library using red fluorescent dyes. Presence of positive and false positive beads 
260 |c 2009 
270 1 0 |m Camperi, S. A.; Cátedra de Microbiología Industrial y Biotecnología, Facultad de Farmacia y Bioquímica, Universidad de Buenos Aires, Junín 956, (1113) Ciudad Autónoma de Buenos Aires, Argentina; email: scamperi@yahoo.com 
506 |2 openaire  |e Política editorial 
504 |a The following abbreviations are used: ACN, acetonitrile; AcOH, acetic acid; BSA, bovine serum albumin; BSA-TR, bovine serum albumin-Texas Red; CHCA, α-cyano-4-hydroxycinnamic acid; DCM, dichloromethane; DIPCDI, N, N-1,3-diisopropylcarbodiimide; DIPEA, N,N-diisopropylethylamine; DMAP, 4-(N,N-dimefhylamino)pyridine; DMF, N,N-dimethylformamide; FITC, fluorescein isothiocyanate; Fmoc-amino acids, fluorenylmethoxyearbonylamino acids; HMBA, 4-hydroxymethylbenzoic acid; HOBt, 1-hydroxybenzotriazole; MALDI-TOF MS, matrix-assisted laser desorption ionization time-of-flight mass spectrometry; OBOC, one-bead one-compound; PBS, phosphate-buffered saline; PEG, poly(ethyleneglycol, SA, streptavidin; SA-ATTO, streptavidin ATTO 590 conjugate; SA-POD, streptavidin peroxidase conjugate; SA-TR, streptavidin Texas red conjugate; TBS, Tris buffer saline; TBTU, 1-[bis(dimethylamino)methylene]-1H-benzotriazolium hexafluorophosphate N-oxide; TFA, triflouroaceti; Lam, K.S., Salmon, S.E., Hersh, E.M., Hruby, V.T., Kazmierski, W.M., Knapp, R.J., (1991) Nature, 354, pp. 82-84 
504 |a Lam, K.S., Hruby, V.J., Lebl, M., (1993) Bioorg. Med. Chem. Lett, 3, pp. 419-244 
504 |a Liu, R., Enstrom, A.M., Lam, K.S., (2003) Exp. Hematol, 31, pp. 11-30 
504 |a Aina, O.H., Liu, R., Sutcliffe, J.L., Marik, J., Pan, C.X., Lam, K.S., (2007) Mol. Pharm, 4, pp. 631-651 
504 |a Camperi, S.A., Iannucci, N.B., Albanesi, G.J., Oggero Eberhardt, M., Etcheverrigaray, M., Messeguer, A., Albericio, F., Cascone, O., (2003) Biotechnol. Lett, 25, pp. 1545-1548 
504 |a Wang, G., De, J., Schoeniger, J.S., Roe, D.C., Carbonell, R.G., (2004) J. Pept. Res, 64, pp. 51-64 
504 |a Lam, K.S., Lehman, A.L., Song, A., Doan, N., Enstrom, A.M., Maxwell, J., Liu, R., Synthesis and screening of "one-bead one-compound" peptide libraries (2003) Methods in Enzymology, 369, pp. 298-322. , Morales, G. A, Bunin, B. A, Eds, Academic Press: New York 
504 |a Camperi, S.A., Marani, M.M., Iannucci, N.B., Côté, S., Albericio, F., Cascone, O., (2005) Tetrahedron Lett, 46, pp. 1561-1564 
504 |a Marani, M.M., Oliveira, E., Côté, S., Camperi, S.A., Albericio, F., Cascone, O., (2007) Anal. Biochem, 370, pp. 215-222 
504 |a Lam, K.S., Lebl, M., (1992) Immunomethods, 1, pp. 11-15 
504 |a Kodadek, T., Bachhawat-Sikder, K., (2006) Mol. Biosyst, 2, pp. 25-35 
504 |a http://www.atto-tec.com/ATTO-TEC.com, ATTO-TEC GmbH, accessed March 2007; Invitrogen, , http://probes.invitrogen.com/handbook, accessed June 2008 
504 |a Côté, S., International Publication (2005), no. WO/01277. Int. Patent Appl. PCT/cd 2004//001464, 2004; Karas, M., Hillenkamp, F., (1988) Anal. Chem, 60, pp. 2299-3201 
504 |a Rozinov, M.N., Nolan, G.P., (1998) Chem. Biol, 5, pp. 713-728 
504 |a Hu, B., Ritter Jones, M., Messersmith, P.B., (2007) Anal. Chem, 79, pp. 7275-7285 
504 |a García-Martín, F., Quintanar-Audelo, M., García-Ramos, Y., Cruz, L.J., Gravel, C., Furic, R., Côté, S., Albericio, F., (2006) J. Comb. Chem, 8, pp. 213-220 
504 |a Axelrod, D., Hellen, E. H. Fulbright, R. M. Total internal reflection fluorescence. In Topics in Fluorescence Spectroscopy, 3. Biochemical Applications; Lakowicz, J. R., Ed.; Plenum Press: New York, 1991; pp 289-344; Mellor, S.L., Wellings, D.A., Fehrentz, J.A., Paris, M., Martinez, J., Ede, N.J., Bray, A.M., Bloomberg, G.B., Synthesis of modified peptides (2000) Fmoc Solid Phase Peptide Synthesis. A Practical Approach, pp. 137-181. , Chan, W. C, White, P. D. Eds, Oxford University Press: New York 
504 |a Brav, A.M., Valerio, R.M., Maeji, N.J., (1993) Tetrahedron Lett, 4, pp. 4411-4414 
504 |a http://www.unionbio.com, Union Biometrica, accessed 2007; Christensen, C.; Groth, T.; Schiødt, C. B.; Foged, N. T.; Meldal, M. OSAR Comb. Sci. 2003, 22, 737-744 
520 3 |a To screen one-bead-one-compound (OBOC) combinatorial libraries, tens of thousands to millions of compound beads are first mixed with a target molecule. The beads that interact with this molecule are then identified and isolated for compound structure determination. Here we describe an OBOC peptide library screening using streptavidin (SA) as probe protein, labeled with a red fluorescent dye and using the COPAS BIO-BEAD flow sorting equipment to separate fluorescent from nonfluorescent beads. The red dyes used were ATTO 590 and Texas Red. After incubating the library with the SA-red fluorescent dye conjugate, we isolated positive beads caused by peptide-SA interaction and false positive beads produced by peptide-fluorescent dye interaction. These false positives were a drawback when sorting beads by COPAS. However, an in depth analysis of both kinds of beads allowed the differentiation of positives from false positives. The false positive beads showed bright homogeneous fluorescence, while positive beads had a heterogeneous fluorescence, exhibiting a characteristic halo appearance, with fluorescence intensity greatest at the bead surface and lowest in the core. The difference was more evident when using Texas Red instead of ATTO 590. Thus, positive beads could be manually separated from false positive ones. The beads were analyzed by matrix-assisted laser desorption ionization time-of-flight mass spectrometry (MALDI-TOF MS). Most of the sequences obtained from positive beads had the His-Pro-Gln motif. Peptides from false positive beads were rich in Leu/Ileu, His, Phe, and Tyr. © 2009 American Chemical Society.  |l eng 
593 |a Cátedra de Microbiología Industrial y Biotecnología, Facultad de Farmacia y Bioquímica, Universidad de Buenos Aires, Junín 956, (1113) Ciudad Autónoma de Buenos Aires, Argentina 
593 |a CIHDECAR-CONICET, Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón II-Ciudad Universitaria, (1428) Ciudad Autónoma de Buenos Aires, Argentina 
593 |a Proteomics Platform, Barcelona Science Park, Baldiri Reixac 10, 08028 Barcelona, Spain 
593 |a Matrix Innovation Inc., 945 Newton, Québec City, QC, Canada 
593 |a Institute for Research in Biomedicine, Barcelona Science Park, Baldiri Reixac 10, 08028 Barcelona, Spain 
593 |a CIBER-BBN, Networking Centre on Bioengineering, Biomaterials and Nanomedicine, Barcelona Science Park, Baldiri Reixac 10, 08028 Barcelona, Spain 
690 1 0 |a FLUORESCENT DYE 
690 1 0 |a MICROSPHERE 
690 1 0 |a PEPTIDE LIBRARY 
690 1 0 |a ARTICLE 
690 1 0 |a COMBINATORIAL CHEMISTRY 
690 1 0 |a DRUG SCREENING 
690 1 0 |a METHODOLOGY 
690 1 0 |a COMBINATORIAL CHEMISTRY TECHNIQUES 
690 1 0 |a DRUG EVALUATION, PRECLINICAL 
690 1 0 |a FLUORESCENT DYES 
690 1 0 |a MICROSPHERES 
690 1 0 |a PEPTIDE LIBRARY 
700 1 |a Ceron, M.C.M. 
700 1 |a Giudicessi, S.L. 
700 1 |a De Oliveira, E. 
700 1 |a Côté, S. 
700 1 |a Erra-Balsells, R. 
700 1 |a Albericio, F. 
700 1 |a Cascone, O. 
700 1 |a Camperi, S.A. 
773 0 |d 2009  |g v. 11  |h pp. 146-150  |k n. 1  |p J. Comb. Chem.  |x 15204766  |t Journal of Combinatorial Chemistry 
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856 4 0 |u https://doi.org/10.1021/cc800145c  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_15204766_v11_n1_p146_Marani  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_15204766_v11_n1_p146_Marani  |y Registro en la Biblioteca Digital 
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999 |c 69943