A specific heat anomaly in multiwall carbon nanotubes as a possible sign of orientational order-disorder transition
We present micro-calorimetric specific heat measurements on different multiwall carbon nanotubes of large outer diameter, as a function of temperature in the range 10-120 K. A clear anomaly at 60 K with the shape of a peak is present in two of the samples, and both the height and the characteristic...
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Elsevier Ltd
2010
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| 024 | 7 | |2 scopus |a 2-s2.0-70449534790 | |
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| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Jorge, G.A. | |
| 245 | 1 | 2 | |a A specific heat anomaly in multiwall carbon nanotubes as a possible sign of orientational order-disorder transition |
| 260 | |b Elsevier Ltd |c 2010 | ||
| 270 | 1 | 0 | |m Jorge, G.A.; Laboratorio de Bajas Temperaturas, Departamento de Física, FCEyN-UBA, Pab. 1, Ciudad Universitaria, 1428 Buenos Aires, Argentina; email: gjorge@df.uba.ar |
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| 506 | |2 openaire |e Política editorial | ||
| 520 | 3 | |a We present micro-calorimetric specific heat measurements on different multiwall carbon nanotubes of large outer diameter, as a function of temperature in the range 10-120 K. A clear anomaly at 60 K with the shape of a peak is present in two of the samples, and both the height and the characteristic temperature of the peak are independent of magnetic field and do not exhibit thermal hysteresis, discarding magnetic degrees of freedom related to Fe seeds or contributions from adsorbed gases. These features suggest that the anomaly may be caused by a structural change. As the anomaly is also unaffected by induced intertube disorder, it may be related with a melting of orientational dislocations of individual tubes within multiwall nanotubes, an effect that was theoretically predicted to occur in carbon nanotubes and represents a distinctive feature of asymmetric molecular systems. © 2009 Elsevier Ltd. All rights reserved. |l eng | |
| 536 | |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT2006-01201 | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP5609 | ||
| 536 | |a Detalles de la financiación: This work was supported by CONICET (PIP5609) and ANPCyT (PICT2006-01201). | ||
| 593 | |a Laboratorio de Bajas Temperaturas, Departamento de Física, FCEyN-UBA, Pab. 1, Ciudad Universitaria, 1428 Buenos Aires, Argentina | ||
| 593 | |a Laboratorio de Polímeros y Materiales Compuestos, Departamento de Física, FCEyN-UBA, Pab. 1, Ciudad Universitaria, 1428 Buenos Aires, Argentina | ||
| 593 | |a Departamento de Química Inorgánica, Analítica y Química Física, FCEyN-UBA, Pab. 2, Ciudad Universitaria, 1428 Buenos Aires, Argentina | ||
| 593 | |a PINMATE, Departamento de Industrias, FCEyN-UBA, Pab. Industrias, Ciudad Universitaria, 1428 Buenos Aires, Argentina | ||
| 593 | |a Instituto de Fisicoquímica de Materiales, Ambiente y Energía, CONICET-UBA, Ciudad Universitaria, 1428 Buenos Aires, Argentina | ||
| 690 | 1 | 0 | |a DEGREES OF FREEDOM (MECHANICS) |
| 690 | 1 | 0 | |a ORDER DISORDER TRANSITIONS |
| 690 | 1 | 0 | |a SPECIFIC HEAT |
| 690 | 1 | 0 | |a THERMAL VARIABLES MEASUREMENT |
| 690 | 1 | 0 | |a YARN |
| 690 | 1 | 0 | |a ADSORBED GAS |
| 690 | 1 | 0 | |a CHARACTERISTIC TEMPERATURE |
| 690 | 1 | 0 | |a MOLECULAR SYSTEMS |
| 690 | 1 | 0 | |a MULTIWALL NANOTUBES |
| 690 | 1 | 0 | |a ORIENTATIONAL ORDERINGS |
| 690 | 1 | 0 | |a OUTER DIAMETERS |
| 690 | 1 | 0 | |a THERMAL HYSTERESIS |
| 690 | 1 | 0 | |a MULTIWALLED CARBON NANOTUBES (MWCN) |
| 700 | 1 | |a Bekeris, V. | |
| 700 | 1 | |a Escobar, M.M. | |
| 700 | 1 | |a Goyanes, Silvia Nair | |
| 700 | 1 | |a Zilli, D. | |
| 700 | 1 | |a Cukierman, A.L. | |
| 700 | 1 | |a Candal, R.J. | |
| 773 | 0 | |d Elsevier Ltd, 2010 |g v. 48 |h pp. 525-530 |k n. 2 |p Carbon |x 00086223 |w (AR-BaUEN)CENRE-4114 |t Carbon | |
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