Antiproliferative terpenoids and alkaloids from the roots of Maytenus vitis-idaea and Maytenus spinosa

Investigation of the organic extracts of the roots of Maytenus vitis-idaea and Maytenus spinosa, collected in the province of Salta, Argentina, led to isolation of eighteen compounds belonging to several classes. From M. vitis-idaea, eight methylenequinone celastroids (1-8) were isolated, four of wh...

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Autor principal: De Almeida, M.T.R
Otros Autores: Ríos-Luci, C., Padrón, J.M, Palermo, J.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2010
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Acceso en línea:Registro en Scopus
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024 7 |2 scopus  |a 2-s2.0-77956344209 
024 7 |2 cas  |a Alkaloids; Antineoplastic Agents, Phytogenic; Sesquiterpenes; Triterpenes 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a PYTCA 
100 1 |a De Almeida, M.T.R. 
245 1 0 |a Antiproliferative terpenoids and alkaloids from the roots of Maytenus vitis-idaea and Maytenus spinosa 
260 |c 2010 
270 1 0 |m Palermo, J. A.; Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón 2, 1428 Buenos Aires, Argentina; email: palermo@qo.fcen.uba.ar 
506 |2 openaire  |e Política editorial 
504 |a Alvarenga, N., Ferro, E.A., Bioactive triterpenes and related compounds from Celastraceae (2006) Stud. Nat. Prod. Chem., 33, pp. 239-307 
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504 |a De Souza E Silva, S.R., De Fátima Silva, G.D., De Almeida Barbosa, L.C., Duarte, L.P., Vieira Filho, S.A., Lupane pentacyclic triterpenes isolated from stems and branches of Maytenus imbricata (Celastraceae) (2005) Helv. Chim. Acta, 88, pp. 1102-1109 
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504 |a González, A.G., Alvarenga, N.L., Ravelo, A.G., Bazzocchi, I.L., Ferro, E.A., Navarro, A.G., Moujir, L., Scutione, a new bioactive norquinonemethide triterpene from Maytenus scutioides (Celastraceae) (1996) Bioorg. Med. Chem., 4, pp. 815-820 
504 |a González, A.G., Alvarenga, N.L., Bazzocchi, I.L., Ravelo, A.G., Moujir, L., Triterpene trimers from Maytenus scutioides: Cycloaddition compounds? (1999) J. Nat. Prod., 62, pp. 1185-1187 
504 |a González, A.G., Bazzocchi, I.L., Moujir, L.M., Jiménez, I.A., Ethnobotanical uses of the Celastraceae (2000) Bioactive Metabolites, Studies in Natural Products Chemistry, 23, pp. 649-738 
504 |a Gunatilaka, A.A.L., Triterpenoid quinonemethides and related compounds (Celastroloids) (1996) Progress in the Chemistry of Organic Natural Products, 67. , Springer Wien New York 
504 |a Gunatilaka, A.A.L., 1H and 13C NMR analysis of three quinone-methide triterpenoids (2005) Magn. Res. Chem., 27, pp. 803-807 
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504 |a Harada, R., Kakisawa, K., Kobayashi, S., Musya, M., Nakanishi, K., Takahashi, Y., Structure of pristimerin, a quinoid triterpene (1962) Tetrahedron Lett., pp. 603-607 
504 |a Miranda, P.O., Padrón, J.M., Padrón, J.I., Villar, J., Martín, V.S., Prins-type synthesis and SAR study of cytotoxic alkyl chloro dihydropyrans (2006) ChemMedChem, 1, pp. 323-329 
504 |a Monks, A., Scudiero, D.A., Skehan, P., Shoemaker, R.H., Paull, K.D., Vistica, D.T., Hose, C., Mayo, M.R., Feasibility of a high-flux anticancer drug screen using a diverse panel of cultured human tumor cell lines (1991) J. Natl. Cancer Inst., 83, pp. 757-766 
504 |a Muñoz, O., Penaloza, A., Gonzalez, A.G., Ravelo, A.G., Bazzocchi, I.L., Alvarenga, N.L., The Celastraceae from Latin America, chemistry and biological activity (1995) Stud. Nat. Prod. Chem., 18, pp. 739-783 
504 |a Nakanishi, K., Kakisawa, H., Hirata, Y., Structure of pristimerin and celastrol (1955) J. Am. Chem. Soc., 77, pp. 3169-3171 
504 |a Ngassapa, O., Soejarto, D., Pezzuto, J., Farnsworth, N., Quinone methide triterpenes and salaspermic acid from Kokoona ochracea (1994) J. Nat. Prod., 57, pp. 1-8 
504 |a Ravelo, A.G., Estévez-Braun, A., Chávez-Orellana, H., Pérez-Sacau, E., Mesa-Siverio, D., Recent studies on natural products as anticancer agents (2004) Curr. Top. Med. Chem., 4, pp. 241-265 
504 |a Shirota, O., Morita, H., Takeya, K., Itokawa, H., Sesquiterpene pyridine alkaloids from Maytenus ilicifolia (1994) Heterocycles, 38, pp. 383-389 
504 |a Shirota, O., Morita, H., Takeya, K., Itokawa, H., New geometric and stereoisomeric triterpene dimers from Maytenus chuchuhuasca (1998) Chem. Pharm. Bull., 46, pp. 102-106 
504 |a Simmons, M.P., Cappa, J., Archer, R., Ford, A.J., Eichstedt, D., Clevinger, C., Phylogeny of the Celastreae (Celastraceae) and the relationships of Catha edulis (qat) inferred from morphological characters and nuclear and plastid genes (2008) Mol. Phylogenet. Evol., 48, pp. 745-757 
504 |a Sugiura, K., Yamada, K., Hirata, Y., The structures of evonimine and euonine, two minor alkaloids obtained from Euonymus sieboldiana Blume (1973) Tetrahedron Lett., pp. 113-116 
520 3 |a Investigation of the organic extracts of the roots of Maytenus vitis-idaea and Maytenus spinosa, collected in the province of Salta, Argentina, led to isolation of eighteen compounds belonging to several classes. From M. vitis-idaea, eight methylenequinone celastroids (1-8) were isolated, four of which (4-7) were hitherto unknown. Additionally, from M. spinosa, two known celastroids, a known celastroid dimer (9), three pentacyclic triterpenoids (10-12) and six β-dihydroagarofuran sesquiterpenoid alkaloids (13-18) were identified. Compounds 4-7 were active against six solid tumor cell lines at micromolar concentrations. © 2010 Elsevier Ltd. All rights reserved.  |l eng 
536 |a Detalles de la financiación: Universidad de Buenos Aires 
536 |a Detalles de la financiación: Coordenação de Aperfeiçoamento de Pessoal de Nível Superior 
536 |a Detalles de la financiación: Umweltbundesamt 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT, 14321 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PEI 6478 
536 |a Detalles de la financiación: We thank Prof. Juan Carlos Oberti and Dr. Viviana Nicotra (Universidad de Córdoba) for encouraging this work, collecting the plant material and providing the extracts, and Prof. Angel Gutiérrez Ravelo (IUBO, Universidad de La Laguna, Tenerife, Spain) for mass spectra, reference NMR spectra, and helpful suggestions. We also thank Mg. Laura Patiño Cano, Mr. José Gallardo and Lic. Gernot Eskuche (UMYMFOR–CONICET) for technical assistance. Research at the University of Buenos Aires was supported by grants from CONICET (PEI 6478), UBA (X 260 Programación 2004–2007), and ANPCyT (PICT (2003) 14321). Research at the University of La Laguna was co-financed by the EU FEDER: the Spanish MICIIN (CTQ2008-06806-C02-01/BQU) and MSC (RTICC RD06/0020/1046); the Canary Islands ACIISI (PI 2007/021) and FUNCIS (PI 01/06 and 35/06). J.M.P. thanks the Spanish MEC-FSE for a Ramón y Cajal contract. M.T.R. de A. thanks CAPES (Brazil) for a doctoral fellowship. Appendix A 
593 |a Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón 2, 1428 Buenos Aires, Argentina 
593 |a BioLab, Instituto Universitario de Bio-Orgánica Antonio González (IUBO-AG), Universidad de la Laguna, Spain 
593 |a Departamento de Ciências Farmacêuticas, Universidade Federal de Santa Catarina, Campus Trindade, 88040-970 Florianópolis, SC, Brazil 
690 1 0 |a Β-DIHYDROAGAROFURAN SESQUITERPENOID ALKALOIDS 
690 1 0 |a CELASTRACEAE 
690 1 0 |a CELASTROIDS 
690 1 0 |a MAYTENUS SPINOSA 
690 1 0 |a MAYTENUS VITIS-IDAEA 
690 1 0 |a METHYLENEQUINONE 
690 1 0 |a PENTACYCLIC TRITERPENOIDS 
690 1 0 |a ALKALOID 
690 1 0 |a ANTINEOPLASTIC AGENT 
690 1 0 |a SESQUITERPENE 
690 1 0 |a TRITERPENE 
690 1 0 |a ARTICLE 
690 1 0 |a CHEMICAL STRUCTURE 
690 1 0 |a CHEMISTRY 
690 1 0 |a DOSE RESPONSE 
690 1 0 |a DRUG SCREENING 
690 1 0 |a HELA CELL 
690 1 0 |a HUMAN 
690 1 0 |a ISOLATION AND PURIFICATION 
690 1 0 |a MAYTENUS 
690 1 0 |a MEDICINAL PLANT 
690 1 0 |a NUCLEAR MAGNETIC RESONANCE 
690 1 0 |a PLANT ROOT 
690 1 0 |a ALKALOIDS 
690 1 0 |a ANTINEOPLASTIC AGENTS, PHYTOGENIC 
690 1 0 |a DOSE-RESPONSE RELATIONSHIP, DRUG 
690 1 0 |a DRUG SCREENING ASSAYS, ANTITUMOR 
690 1 0 |a HELA CELLS 
690 1 0 |a HUMANS 
690 1 0 |a MAYTENUS 
690 1 0 |a MOLECULAR STRUCTURE 
690 1 0 |a NUCLEAR MAGNETIC RESONANCE, BIOMOLECULAR 
690 1 0 |a PLANT ROOTS 
690 1 0 |a PLANTS, MEDICINAL 
690 1 0 |a SESQUITERPENES 
690 1 0 |a TRITERPENES 
690 1 0 |a CELASTRACEAE 
690 1 0 |a IDAEA 
690 1 0 |a MAYTENUS 
690 1 0 |a VITACEAE 
690 1 0 |a VITIS 
651 4 |a ARGENTINA 
651 4 |a ARGENTINA 
700 1 |a Ríos-Luci, C. 
700 1 |a Padrón, J.M. 
700 1 |a Palermo, J.A. 
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