Binding of Pb(II) in the system humic acid/goethite at acidic pH
The study of Pb(II) binding to the system humic acid/goethite in acidic medium is reported in the present paper. From a macroscopic point of view, we have constructed the experimental sorption isotherms (using atomic absorption spectroscopy) and compared them with the prediction of the additivity ru...
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2006
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| LEADER | 13159caa a22014777a 4500 | ||
|---|---|---|---|
| 001 | PAPER-6845 | ||
| 003 | AR-BaUEN | ||
| 005 | 20230518203634.0 | ||
| 008 | 190411s2006 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-33751018872 | |
| 024 | 7 | |2 cas |a ferric hydroxide, 11113-66-9, 12022-37-6, 12181-28-1, 1309-33-7, 1310-14-1, 1317-60-8, 1317-63-1; humic acid, 1415-93-6; lead, 7439-92-1; oxide, 16833-27-5; proton, 12408-02-5, 12586-59-3; goethite, 1310-14-1; Humic Substances; Iron Compounds; Lead, 7439-92-1 | |
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 030 | |a CMSHA | ||
| 100 | 1 | |a Orsetti, S. | |
| 245 | 1 | 0 | |a Binding of Pb(II) in the system humic acid/goethite at acidic pH |
| 260 | |c 2006 | ||
| 270 | 1 | 0 | |m Andrade, E.M.; INQUIMAE, DQIAQF, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria Pabellon II, 1428 Buenos Aires, Argentina; email: eandrade@qi.fcen.uba.ar |
| 506 | |2 openaire |e Política editorial | ||
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| 520 | 3 | |a The study of Pb(II) binding to the system humic acid/goethite in acidic medium is reported in the present paper. From a macroscopic point of view, we have constructed the experimental sorption isotherms (using atomic absorption spectroscopy) and compared them with the prediction of the additivity rule. It is found that this system presents positive deviations, that is, the amount sorbed is about an order of magnitude higher than predicted. Apart from this, microscopic and structural aspects have also been studied using in situ and ex situ infrared spectroscopy. These results suggest that the presence of Pb(II) increases the amount of humic acid bound to the oxide. It is proposed that proton displacement due to the interaction between humic substances and the oxide, along with the formation of ternary complexes with the Pb(II) cation bridging the oxide and the humic substances (Type A complexes), cause the deviation from additivity. © 2006 Elsevier Ltd. All rights reserved. |l eng | |
| 536 | |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, 06-12467 | ||
| 536 | |a Detalles de la financiación: Universidad de Buenos Aires, UBACYT 2004–2007 X105 | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP 02287 | ||
| 536 | |a Detalles de la financiación: The authors gratefully acknowledge financial support from the Universidad de Buenos Aires (UBACYT 2004–2007 X105), the Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET, PIP 02287) and the Agencia Nacional de Promoción Científica y Tecnológica (grant No. 06-12467). The authors wish to thank Dr. Jorge Stripeikis for his kind help with the AAS measurements as well as Dr. Roberto Candal for kindly supplying the goethite samples used in this work. | ||
| 593 | |a INQUIMAE, DQIAQF, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria Pabellon II, 1428 Buenos Aires, Argentina | ||
| 690 | 1 | 0 | |a METAL POLLUTION |
| 690 | 1 | 0 | |a MULTISUBSTRATE ADSORPTION |
| 690 | 1 | 0 | |a OXIDE-HUMATE-METAL COMPLEX |
| 690 | 1 | 0 | |a SOIL CHEMISTRY |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ADSORPTION ISOTHERMS |
| 690 | 1 | 0 | |a COMPLEXATION |
| 690 | 1 | 0 | |a INFRARED SPECTROSCOPY |
| 690 | 1 | 0 | |a LEAD |
| 690 | 1 | 0 | |a ORGANIC ACIDS |
| 690 | 1 | 0 | |a METAL POLLUTION |
| 690 | 1 | 0 | |a MULTISUBSTRATE ADSORPTION |
| 690 | 1 | 0 | |a OXIDE-HUMATE-METAL COMPLEX |
| 690 | 1 | 0 | |a SOIL CHEMISTRY |
| 690 | 1 | 0 | |a SOIL POLLUTION |
| 690 | 1 | 0 | |a CATION |
| 690 | 1 | 0 | |a FERRIC HYDROXIDE |
| 690 | 1 | 0 | |a HUMIC ACID |
| 690 | 1 | 0 | |a LEAD |
| 690 | 1 | 0 | |a OXIDE |
| 690 | 1 | 0 | |a PROTON |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ADSORPTION ISOTHERMS |
| 690 | 1 | 0 | |a COMPLEXATION |
| 690 | 1 | 0 | |a INFRARED SPECTROSCOPY |
| 690 | 1 | 0 | |a LEAD |
| 690 | 1 | 0 | |a ORGANIC ACIDS |
| 690 | 1 | 0 | |a SOIL POLLUTION |
| 690 | 1 | 0 | |a GOETHITE |
| 690 | 1 | 0 | |a HUMIC ACID |
| 690 | 1 | 0 | |a LEAD |
| 690 | 1 | 0 | |a OXIDE |
| 690 | 1 | 0 | |a SOIL CHEMISTRY |
| 690 | 1 | 0 | |a SOIL POLLUTION |
| 690 | 1 | 0 | |a SORPTION |
| 690 | 1 | 0 | |a ACIDITY |
| 690 | 1 | 0 | |a ARTICLE |
| 690 | 1 | 0 | |a ATOMIC ABSORPTION SPECTROMETRY |
| 690 | 1 | 0 | |a COMPARATIVE STUDY |
| 690 | 1 | 0 | |a INFRARED SPECTROSCOPY |
| 690 | 1 | 0 | |a METAL BINDING |
| 690 | 1 | 0 | |a PREDICTION |
| 690 | 1 | 0 | |a SOIL POLLUTION |
| 690 | 1 | 0 | |a HUMIC SUBSTANCES |
| 690 | 1 | 0 | |a HYDROGEN-ION CONCENTRATION |
| 690 | 1 | 0 | |a IRON COMPOUNDS |
| 690 | 1 | 0 | |a LEAD |
| 690 | 1 | 0 | |a SPECTROPHOTOMETRY, INFRARED |
| 690 | 1 | 0 | |a SPECTROPHOTOMETRY, ULTRAVIOLET |
| 690 | 1 | 0 | |a SPECTROSCOPY, FOURIER TRANSFORM INFRARED |
| 650 | 1 | 7 | |2 spines |a PH |
| 650 | 1 | 7 | |2 spines |a PH |
| 700 | 1 | |a de las Mercedes Quiroga, M. | |
| 700 | 1 | |a Andrade, E.M. | |
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