Thermal properties in cured natural rubber/styrene butadiene rubber blends

Blends of natural rubber (NR) and styrene butadiene rubber (SBR) were prepared with sulfur and n-t-butyl-2-benzothiazole sulfonamide (TBBS) as accelerator, varying the amount of each polymer in the blend. Samples were analysed by rheometer curing at 433 K until their maximum torque was reached. The...

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Autor principal: Goyanes, Silvia Nair
Otros Autores: Lopez, C.C, Rubiolo, Gerardo Héctor, Quasso, F., Marzocca, Angel José
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2008
Acceso en línea:Registro en Scopus
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040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
100 1 |a Goyanes, Silvia Nair 
245 1 0 |a Thermal properties in cured natural rubber/styrene butadiene rubber blends 
260 |c 2008 
270 1 0 |m Marzocca, A.J.; Universidad de Buenos Aires, Facultad de Ciencias Exactas y Naturales, Dto. de Física, Ciudad Universitaria, Pabellon 1, 1428 Buenos Aires, Argentina; email: marzo@df.uba.ar 
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504 |a Murashov, V.V., White, M.A., Apparatus for dynamical thermal measurements of low-thermal diffusivity particulate materials at subambient temperatures (1998) Rev Sci Instrum, 69, pp. 4198-4204 
504 |a Pourppoint, T.L., Banish, R.M., Wessling, F.C., Sekerka, R.F., Real-time determination of thermal diffusivity in a disk-shaped sample: applications to graphite and boron nitride (2000) Rev Sci Instrum, 71, pp. 4512-4520 
504 |a Vozár, L., Groboth, G., Thermal diffusivity measurement of poorly conductive materials: a comparison of step-heating and flash methods (1997) High Temp-High Press, 29, pp. 191-199 
504 |a Kubičár, L., Boháč, V., A step-wise method for measuring thermophysical parameters of materials (2000) Meas Sci Technol, 11, pp. 252-258 
504 |a Mariani, M.C., Beccar Varela, M.P., Marzocca, A.J., An improvement in the determination of thermal properties of elastomeric compounds (1997) Kautsch Gummi Kunstst, 50, pp. 39-42 
504 |a Camaño, E., Martire, N., Goyanes, S.N., Marzocca, A.J., Rubiolo, G.H., Evaluation of thermal diffusivity of rubber compounds through the glass transition range (1997) J Appl Polym Sci, 63, pp. 157-162 
504 |a Goyanes, S.N., Beccar Varela, M.P., Mariani, M.C., Marzocca, A.J., Influence of the carbon black dispersion in the thermal diffusivity of a SBR vulcanizate (1999) J Appl Polym Sci, 72, pp. 1379-1385 
504 |a Goyanes, S.N., Marconi, J.D., König, P.G., Rubiolo, G.H., Matteo, C.L., Marzocca, A.J., Analysis of thermal diffusivity in aluminum (particle) filled PMMA compounds (2002) Polymer, 42, pp. 5267-5274 
504 |a Vilgis, T.A., Heinrich, G., Crosslinked polymer blends: theoretical problems from rubber physics to technology (1995) Kautsch Gummi Kunstst, 48, pp. 323-335 
504 |a Sircar, A.K., (1981) Thermal characterization of polymeric materials, pp. 887-1378. , Turi E.A. (Ed), Academic Press, San Diego 
504 |a Saxena, N.S., Pradeep, P., Mathew, G., Thomas, S., Gustafsson, M., Gustafsson, S.E., Thermal conductivity of styrene butadiene rubber compounds with natural rubber prophylactics waste as filler (1999) Eur Polym J, 35, pp. 1687-1693 
504 |a Beccar Varela MP, Mariani MC, Marzocca AJ, Rial DF. Estimation of the dependence of the elastomer thermal diffusivity with the temperature. In: D'Attellis CE, Fernandez-Berdaguer EM, editors. Proceeding of the first latin American workshop of applied mathematicae in industry and medicine. Buenos Aires: CLAMI; 1996. p. 183-6; Hands, D., Horsfall, F., The thermal diffusivity and conductivity of natural rubber compounds (1977) Rubber Chem Technol, 50, pp. 253-265 
504 |a Ghilarducci, A., Cerveny, S., Salva, H., Matteo, C.L., Marzocca, A.J., Influence of the blend composition the internal friction of NR/SBR compounds (2001) Kautsch Gummi Kunstst, 54, pp. 382-386 
504 |a Hourston, D.J., Song, M., Quantitative characterization of interfaces in rubber-rubber blends by means of modulated-temperature DSC (2000) J Appl Polym Sci, 76, pp. 1791-1798 
504 |a Mallon, P.E., McGill, W.J., Polyisoprene, poly(styrene-cobutadiene), and their blends. I Vulcanization reactions with tetramethylthiuram disulfide/sulfur (1999) J Appl Polym Sci, 74, pp. 1250-1263 
504 |a Mallon, P.E., McGill, W.J., Polyisoprene, poly(styrene-cobutadiene), and their blends. Part II. Vulcanization reactions with 2-bisbezothiazole-2,2′ disulfide/sulfur (1999) J Appl Polym Sci, 74, pp. 1264-1270 
504 |a Mallon, P.E., McGill, W.J., Polyisoprene, poly(styrene-cobutadiene) and their blends. III. Tensile properties of tetramethylthiuram disulfide/sulfur and 2-bisbenzothiazole-2,2′-disulfide/sulfur compounds (1999) J Appl Polym Sci, 74, pp. 2143-2149 
504 |a Shefer, A., Gottlieb, M., Effect of cross-link on the glass transition temperature of end-linked elastomers (1992) Macromolecules, 25, pp. 4036-4042 
504 |a Marzocca, A.J., Steren, C.A., Raimondo, R.B., Cerveny, S., Influence of the cure level on the monomeric friction coefficient of natural rubber vulcanizates (2004) Polym Int, 56, pp. 646-655 
504 |a Gehman, S.D., Heat transfer in processing and use of rubber (1967) Rubber Chem Technol, 40, pp. 36-99 
506 |2 openaire  |e Política editorial 
520 3 |a Blends of natural rubber (NR) and styrene butadiene rubber (SBR) were prepared with sulfur and n-t-butyl-2-benzothiazole sulfonamide (TBBS) as accelerator, varying the amount of each polymer in the blend. Samples were analysed by rheometer curing at 433 K until their maximum torque was reached. The miscibility among the constituent polymers of the cured compounds was studied in a broad range of temperatures by means of differential scanning calorimetry, analyzing the glass transition temperatures of the samples. The specific heat capacity of the compounds was also determined. Thermal diffusivity of the samples was measured in the temperature range from 130 to 400 K with a new device that performs measurements in vacuum. The thermal results are explained on the basis of the structure formed during the vulcanization of the samples considering the variation of the crosslink density of each phase. Finally, a serial thermal conduction model that takes into account the contribution of each phase to the thermal diffusivity was used to fit the experimental results. © 2008 Elsevier Ltd. All rights reserved.  |l eng 
536 |a Detalles de la financiación: Consejo Nacional para Investigaciones Científicas y Tecnológicas 
536 |a Detalles de la financiación: Consejo Nacional para Investigaciones Científicas y Tecnológicas 
536 |a Detalles de la financiación: Universidad de Buenos Aires, X191and X808 
536 |a Detalles de la financiación: This work was supported by the Universidad de Buenos Aires, Argentina (Investigation Project X191and X808), Consejo Nacional de Investigaciones Científicas y Tecnológicas (Argentina) and Agencia Nacional de Investigaciones Científicas y Tecnológicas (Argentina). The authors want to thanks Fate SAICI (Argentina) for the preparation of the samples. 
593 |a Universidad de Buenos Aires, Facultad de Ciencias Exactas y Naturales, Dto. de Física, Ciudad Universitaria, Pabellon 1, 1428 Buenos Aires, Argentina 
593 |a Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET), Argentina 
593 |a Departamento de Materiales, CNEA, Av. del Libertador 8250, 1424 Buenos Aires, Argentina 
593 |a Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano, Italy 
690 1 0 |a GLASS TRANSITION TEMPERATURE 
690 1 0 |a NR/SBR BLENDS 
690 1 0 |a SPECIFIC HEAT 
690 1 0 |a THERMAL DIFFUSIVITY 
690 1 0 |a VULCANIZATION 
690 1 0 |a AROMATIC POLYMERS 
690 1 0 |a CROSSLINKING 
690 1 0 |a DIFFERENTIAL SCANNING CALORIMETRY 
690 1 0 |a GLASS TRANSITION 
690 1 0 |a RHEOLOGY 
690 1 0 |a SOLUBILITY 
690 1 0 |a THERMAL DIFFUSIVITY 
690 1 0 |a VULCANIZATION 
690 1 0 |a N-T-BUTYL-2-BENZOTHIAZOLE SULFONAMIDE (TBBS) 
690 1 0 |a NR/SBR BLENDS 
690 1 0 |a STYRENE BUTADIENE RUBBER (SBR) 
690 1 0 |a RUBBER 
700 1 |a Lopez, C.C. 
700 1 |a Rubiolo, Gerardo Héctor 
700 1 |a Quasso, F. 
700 1 |a Marzocca, Angel José 
773 0 |d 2008  |g v. 44  |h pp. 1525-1534  |k n. 5  |p Eur Polym J  |x 00143057  |w (AR-BaUEN)CENRE-4697  |t European Polymer Journal 
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