A unique family of stable and water-soluble S-nitrosothiol complexes

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In this work, we present a complete and detailed experimental characterization and theoretical study of a variety of coordinated S-nitrosothiols (RSNOs), such as cysteine derivatives, mercaptosuccinic acid, benzyl thiol, and phenyl thiol. Some of them are extremely unstable and sensitive in free for...

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Detalles Bibliográficos
Autor principal: Perissinotti, L.L
Otros Autores: Leitus, G., Shimon, L., Estrin, D., Doctorovich, F.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2008
Acceso en línea:Registro en Scopus
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Biblioteca Central Dr. Luis F. Leloir (FCEN) de Universidad de Buenos Aires
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024 7 |2 scopus  |a 2-s2.0-46749120688 
024 7 |2 cas  |a cysteine, 4371-52-2, 52-89-1, 52-90-4; thiomalic acid, 70-49-5; water, 7732-18-5; 2-thiomalic acid, 70-49-5; Cysteine, 52-90-4; Esters; Potassium Compounds; S-Nitrosothiols; Thiomalates; Water, 7732-18-5 
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030 |a INOCA 
100 1 |a Perissinotti, L.L. 
245 1 2 |a A unique family of stable and water-soluble S-nitrosothiol complexes 
260 |c 2008 
270 1 0 |m Doctorovich, F.; Departamento de Quimica Inorganica, Analitica Y Quimica Fisica/INQUIMAE, Facultad de Ciencias Exactas Y Naturales, Pabellón II, (C1428EHA) Buenos Aires, Argentina; email: doctorovich@qi.fcen.uba.ar 
506 |2 openaire  |e Política editorial 
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504 |a Perissinotti, L.L., Estrin, D.A., Leitus, G., Doctorovich, F., (2006) J. Am. Chem. Soc, 128 (8), pp. 2512-2513 
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504 |a Doctorovich, F., Di Salvo, F., Escola, N., Trapani, C., Shimon, L., (2005) Organometallics, 24 (20), pp. 4707-4709 
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520 3 |a In this work, we present a complete and detailed experimental characterization and theoretical study of a variety of coordinated S-nitrosothiols (RSNOs), such as cysteine derivatives, mercaptosuccinic acid, benzyl thiol, and phenyl thiol. Some of them are extremely unstable and sensitive in free form. Strikingly, in contrast with free S-nitrosothiols, we found that, upon coordination to iridium, they become very stable even in aqueous solutions. The study of these coordinated complexes provides further insight on the elucidation of structural aspects dealing with the nature of the S-N bond in RSNOs, a fact which still remains a matter of controversy. © 2008 American Chemical Society.  |l eng 
593 |a Departamento de Quimica Inorganica, Analitica Y Quimica Fisica/INQUIMAE, Facultad de Ciencias Exactas Y Naturales, Pabellón II, (C1428EHA) Buenos Aires, Argentina 
593 |a Department of Chemical Services, Weizmann Institute of Science, Rehovot 76100, Israel 
690 1 0 |a 2 THIOMALIC ACID 
690 1 0 |a 2-THIOMALIC ACID 
690 1 0 |a CYSTEINE 
690 1 0 |a ESTER 
690 1 0 |a POTASSIUM DERIVATIVE 
690 1 0 |a S NITROSOTHIOL 
690 1 0 |a THIOMALIC ACID 
690 1 0 |a WATER 
690 1 0 |a ARTICLE 
690 1 0 |a CHEMISTRY 
690 1 0 |a ELECTROSPRAY MASS SPECTROMETRY 
690 1 0 |a INFRARED SPECTROSCOPY 
690 1 0 |a NUCLEAR MAGNETIC RESONANCE SPECTROSCOPY 
690 1 0 |a SOLUBILITY 
690 1 0 |a ULTRAVIOLET SPECTROPHOTOMETRY 
690 1 0 |a X RAY CRYSTALLOGRAPHY 
690 1 0 |a CRYSTALLOGRAPHY, X-RAY 
690 1 0 |a CYSTEINE 
690 1 0 |a ESTERS 
690 1 0 |a MAGNETIC RESONANCE SPECTROSCOPY 
690 1 0 |a POTASSIUM COMPOUNDS 
690 1 0 |a S-NITROSOTHIOLS 
690 1 0 |a SOLUBILITY 
690 1 0 |a SPECTROMETRY, MASS, ELECTROSPRAY IONIZATION 
690 1 0 |a SPECTROPHOTOMETRY, ULTRAVIOLET 
690 1 0 |a SPECTROSCOPY, FOURIER TRANSFORM INFRARED 
690 1 0 |a THIOMALATES 
690 1 0 |a WATER 
700 1 |a Leitus, G. 
700 1 |a Shimon, L. 
700 1 |a Estrin, D. 
700 1 |a Doctorovich, F. 
773 0 |d 2008  |g v. 47  |h pp. 4723-4733  |k n. 11  |p Inorg. Chem.  |x 00201669  |w (AR-BaUEN)CENRE-60  |t Inorganic Chemistry 
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856 4 0 |u https://doi.org/10.1021/ic7024999  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_00201669_v47_n11_p4723_Perissinotti  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_00201669_v47_n11_p4723_Perissinotti  |y Registro en la Biblioteca Digital 
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