Diffusion-viscosity decoupling in supercooled aqueous trehalose solutions
The diffusional mobility of disodium fluorescein has been measured in supercooled aqueous solutions of trehalose, a widely used cryoprotectant disaccharide. The results were analyzed on the basis of the classical continuum hydrodynamic theory (Stokes - Einstein relationship) and compared with result...
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American Chemical Society
2008
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
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| LEADER | 09173caa a22012377a 4500 | ||
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| 001 | PAPER-5648 | ||
| 003 | AR-BaUEN | ||
| 005 | 20250623093704.0 | ||
| 008 | 190411s2008 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-55149115172 | |
| 030 | |a JPCBF | ||
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Corti, H.R. | |
| 245 | 1 | 0 | |a Diffusion-viscosity decoupling in supercooled aqueous trehalose solutions |
| 260 | |b American Chemical Society |c 2008 | ||
| 270 | 1 | 0 | |m Corti, H. R.; Departamento Física de Materia Condensada, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. General Paz 1499, 1650 San Martín, Argentina; email: hrcorti@cnea.gov.ar |
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| 506 | |2 openaire |e Política editorial | ||
| 520 | 3 | |a The diffusional mobility of disodium fluorescein has been measured in supercooled aqueous solutions of trehalose, a widely used cryoprotectant disaccharide. The results were analyzed on the basis of the classical continuum hydrodynamic theory (Stokes - Einstein relationship) and compared with results for the diffusion and electrical conductivity of other ionic and nonionic solutes in trehalose and sucrose aqueous solutions. Disodium fluorescein obeys the classical model over a restricted range of inverse reduced temperatures, Tg/T, scaled by the glass transition temperature. Decoupling in neutral solutes takes place at higher values of Tg/T, while in ionic solutes it occurs all over the range of Tg/T studied, as observed for the water mobility in supercooled sugar solutions. © 2008 American Chemical Society. |l eng | |
| 593 | |a Departamento Física de Materia Condensada, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. General Paz 1499, 1650 San Martín, Argentina | ||
| 593 | |a Institute de Química Física de Materiales, Ambiente y Energía (INQUIMAE), Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Pabellón II, Buenos Aires, Argentina | ||
| 593 | |a Laboratorio de Electrónica Cuántica, Departamento de Física, Ciudad Universitaria, Pabellón I, Buenos Aires, Argentina | ||
| 593 | |a NSF ERC for Extreme Ultraviolet Science and Technology, Department of Electrical and Computer Engineering, Colorado State University, Fort Collins, CO 80525, United States | ||
| 690 | 1 | 0 | |a ELECTRIC CONDUCTIVITY |
| 690 | 1 | 0 | |a FLUID DYNAMICS |
| 690 | 1 | 0 | |a GLASS TRANSITION |
| 690 | 1 | 0 | |a HYDRODYNAMICS |
| 690 | 1 | 0 | |a IONIZATION OF LIQUIDS |
| 690 | 1 | 0 | |a POLYSACCHARIDES |
| 690 | 1 | 0 | |a SEMICONDUCTOR DOPING |
| 690 | 1 | 0 | |a SUGAR (SUCROSE) |
| 690 | 1 | 0 | |a SUGARS |
| 690 | 1 | 0 | |a SUPERCOOLING |
| 690 | 1 | 0 | |a AQUEOUS SOLUTIONS |
| 690 | 1 | 0 | |a CLASSICAL MODELS |
| 690 | 1 | 0 | |a CRYOPROTECTANT |
| 690 | 1 | 0 | |a DIFFUSIONAL MOBILITIES |
| 690 | 1 | 0 | |a ELECTRICAL CONDUCTIVITIES |
| 690 | 1 | 0 | |a GLASS TRANSITION TEMPERATURES |
| 690 | 1 | 0 | |a HYDRODYNAMIC THEORIES |
| 690 | 1 | 0 | |a IONIC SOLUTES |
| 690 | 1 | 0 | |a NONIONIC SOLUTES |
| 690 | 1 | 0 | |a SUGAR SOLUTIONS |
| 690 | 1 | 0 | |a TREHALOSE SOLUTIONS |
| 690 | 1 | 0 | |a WATER MOBILITIES |
| 690 | 1 | 0 | |a SOLUTIONS |
| 700 | 1 | |a Frank, Guillermo Alberto | |
| 700 | 1 | |a Marconi, Mario Carlos | |
| 773 | 0 | |d American Chemical Society, 2008 |g v. 112 |h pp. 12899-12906 |k n. 41 |p J Phys Chem B |x 15206106 |w (AR-BaUEN)CENRE-5879 |t Journal of Physical Chemistry B | |
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