Hydrogen from steam reforming of ethanol. characterization and performance of copper-nickel supported catalysts

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The effect of the copper loading and calcination temperature on the structure and performance of Cu/Ni|K|γ-Al2O3 catalysts is examined. TPR, XRD and N2O chemisorption techniques are employed. Activity and selectivity measurements are carried out considering steam reforming of ethanol as the test rea...

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Detalles Bibliográficos
Autor principal: Mariño, F.J
Otros Autores: Cerrella, E.G, Duhalde, Stella Maris, Jobbagy, M., Laborde, M.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Elsevier Ltd 1998
Acceso en línea:Registro en Scopus
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Biblioteca Central Dr. Luis F. Leloir (FCEN) de Universidad de Buenos Aires
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040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
100 1 |a Mariño, F.J. 
245 1 0 |a Hydrogen from steam reforming of ethanol. characterization and performance of copper-nickel supported catalysts 
260 |b Elsevier Ltd  |c 1998 
270 1 0 |m Mariño, F.J.; Depto. de Ing. Química (FI), Universidad de Buenos Aires, Ciudad Universitaria, 1428 Buenos Aires, Argentina 
504 |a Newsome, D., (1980) Catal. Rev. Sci. Engng., 21, p. 275 
504 |a García, E., Laborde, M., (1991) Int. J. Hydrogen Energy, 16 (5), p. 307 
504 |a Luengo, C., Ciampi, G., Steckelberg, C., Laborde, M., (1992) Int. J. Hydrogen Energy, 17 (9), p. 677 
504 |a Cerrella, E., Duhalde, S., Jobbagy, M., Laborde, M., Mariño, F., (1996) Proceedings First Symposium on Catalysis JICA-CENACA, p. 105. , Santa Fe, Argentina 
504 |a Agarás, H., Cerrela, E., Laborde, M., (1988) Appl. Catal., 45, p. 53 
504 |a Idem, R., Bakshi, N., (1994) Ind. Eng. Chem. Res., 33, p. 2056 
504 |a Osinga, Th., Linsen, B., Van Beek, W., (1967) J. Catal., 7, p. 277 
504 |a Dvorak, B., Pasek, J., (1970) J. Catal., 18, p. 108 
504 |a Evans, J., Wainwright, M., Bridgewater, A., Young, D., (1983) Appl. Cat., 7, p. 75 
504 |a Robertson, S., McNicol, B., De Baas, J., Kloet, S., Jenkins, J., (1975) J. Catal., 37 (3), p. 424 
504 |a Friedman, R., Freeman, J., Lytle, F., (1978) J. Catal., 55, p. 10 
504 |a Hierl, R., Knozinger, H., Urbach, H., (1981) J. Catal., 69, p. 475 
504 |a Strohmeier, B., Leyden, D., Field, R., Hercules, D., (1985) J. Catal., 94 (2), p. 514 
504 |a Robinson, W., Mol, J., (1988) Appl. Cat., 44, p. 165 
504 |a Sivaraj, Ch., Kantarao, P., (1988) Appl. Cat., 45, p. 103 
504 |a Dumas, J., Geron, C., Kribii, A., Barbier, J., (1989) Appl. Cat., 47, pp. L9 
504 |a Pellucchi, N., Cerrella, E., Duhalde, S., Laborde, M., Tejeda, R., (1995) Proceedings VIII Seminário Brasileiro de Catalise, Nova Friburgo - RJ, Brasil, 1, p. 34 
504 |a Ayastuy, J., Gonzalez Velasco, J., Gutierrez Ortiz, M., Laborde, M., (1993) Proceedings VII Seminário Brasileiro de Catalise, Gramado, Brasil, 1, p. 397 
504 |a Giamello, E., Fubini, B., Lauro, P., Bossi, A., (1984) J. Catal., 87, p. 443 
506 |2 openaire  |e Política editorial 
520 3 |a The effect of the copper loading and calcination temperature on the structure and performance of Cu/Ni|K|γ-Al2O3 catalysts is examined. TPR, XRD and N2O chemisorption techniques are employed. Activity and selectivity measurements are carried out considering steam reforming of ethanol as the test reaction. The appearance of CuO phase depends on copper loading and calcination temperature, whereas NiAl2O4 phase is present in all the analyzed samples. Copper dispersion is favored at lower copper loading. TOF values indicate that steam reforming of ethanol should be a structure-sensitivity reaction, at least under the experimental conditions used in this work. © 1998 International Association for Hydrogen Energy.  |l eng 
536 |a Detalles de la financiación: Universidad de Buenos Aires 
536 |a Detalles de la financiación: To Universidad de Buenos Aires for the financial support. To Mr R. Tejeda for his technical assistance. 
593 |a Depto. de Ing. Química (FI), Universidad de Buenos Aires, Ciudad Universitaria, 1428 Buenos Aires, Argentina 
593 |a PINMATE(FCEyN) CONICET, Universidad de Buenos Aires, Ciudad Universitaria, 1428 Buenos Aires, Argentina 
593 |a Departamento de Física (FI), Universidad de Buenos Aires, Ciudad Universitaria, 1428 Buenos Aires, Argentina 
690 1 0 |a ALUMINA 
690 1 0 |a CALCINATION 
690 1 0 |a CATALYST ACTIVITY 
690 1 0 |a CATALYST SELECTIVITY 
690 1 0 |a CATALYST SUPPORTS 
690 1 0 |a CATALYSTS 
690 1 0 |a CHEMISORPTION 
690 1 0 |a COPPER 
690 1 0 |a ETHANOL FUELS 
690 1 0 |a NICKEL 
690 1 0 |a REFORMING REACTIONS 
690 1 0 |a RENEWABLE ENERGY RESOURCES 
690 1 0 |a STEAM REFORMING 
690 1 0 |a HYDROGEN FUELS 
700 1 |a Cerrella, E.G. 
700 1 |a Duhalde, Stella Maris 
700 1 |a Jobbagy, M. 
700 1 |a Laborde, M.A. 
773 0 |d Elsevier Ltd, 1998  |g v. 23  |h pp. 1095-1101  |k n. 12  |p Int J Hydrogen Energy  |x 03603199  |w (AR-BaUEN)CENRE-5264  |t International Journal of Hydrogen Energy 
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856 4 0 |u https://doi.org/10.1016/S0360-3199(97)00173-0  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_03603199_v23_n12_p1095_Marino  |y Handle 
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999 |c 63776 

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