Steam reforming of glycerol over Ni/Mg/γ-Al 2O 3 catalysts. Effect of calcination temperatures
The aim of this work is to study the catalytic activity of Ni(10%) based catalysts supported over ã-Al 2O 3 modified with Mg (3%) for the steam reforming of glycerol. Catalysts have been prepared by incipient wetness impregnation method; analysing the effect of the calcination temperature of the mod...
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| Formato: | Capítulo de libro |
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2012
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
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| LEADER | 06959caa a22007817a 4500 | ||
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| 001 | PAPER-23352 | ||
| 003 | AR-BaUEN | ||
| 005 | 20240927143529.0 | ||
| 008 | 190411s2012 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-84866056202 | |
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| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Dieuzeide, M.L. | |
| 245 | 1 | 0 | |a Steam reforming of glycerol over Ni/Mg/γ-Al 2O 3 catalysts. Effect of calcination temperatures |
| 260 | |c 2012 | ||
| 270 | 1 | 0 | |m Amadeo, N.; Laboratorio de Procesos Catalíticos, Departamento de Ing. Química, Ciudad Universitaria, 1428 C.A.B.A, Argentina; email: norma@di.fcen.uba.ar |
| 504 | |a Chheda, J.N., Huber, G.W., Dumesic, J.A., Liquid-Phase catalytic processing of biomass-derived oxygenated hydrocarbons to fuels and chemicals (2007) Angew Chem Int Ed, 46, pp. 462-522 | ||
| 504 | |a Adhikari, S., Fernando, S., Haryanto, A., Production of hydrogen by steam reforming of glycerin over alumina-supported metal catalysts (2007) Cat Today, 129, pp. 355-364 | ||
| 504 | |a Czernik, S., French, R., Feik, C., Chornet, E., Hydrogen by catalytic steam reforming of liquid byproducts from biomass thermoconversion processes (2002) Ind Eng Chem Res, 41, pp. 4209-4215 | ||
| 504 | |a Hirai, T., Ikenaga, N., Miyake, T., Suzuki, T., Production of hydrogen by steam reforming of glycerine on ruthenium catalyst (2005) Energy Fuels, 19, pp. 1761-1762 | ||
| 504 | |a Soares, R.R., Simonetti, D.A., Dumesic, J.A., Glycerol as a source for fuels and chemicals by low-temperature catalytic processing (2006) Angew Chem Int Ed, 45, pp. 3982-3985 | ||
| 504 | |a Simonetti, D.A., Kunkes, E.L., Dumesic, J.A., Gas-phase conversion of glycerol to synthesis gas over carbon-supported platinum and platinum-rhenium catalysts (2007) J.Catal, 247, pp. 298-306 | ||
| 504 | |a Kunkes, E.L., Soares, R.R., Simonetti, D.A., Dumesic, J.A., An integrated catalytic approach for the production of hydrogen by glycerol reforming coupled with water-gas shift (2009) Appl Catal. B, 90, pp. 693-698 | ||
| 504 | |a Adhikari, S., Fernando, S.D., Filip To, S.D., Mark Bricka, R., Steele, P.H., Haryanto, A., Conversion of glycerol to hydrogen via a steam reforming process over nickel catalysts (2008) Energy Fuels, 22, pp. 1220-1226 | ||
| 504 | |a Iriondo, A., Barrio, V.L., Cambra, J.F., Arias, P.L., Guemez, M.B., Navarro, R.M., Hydrogen production from glicerol over nickel catalysts supported on Al 2O 3 modified by Mg, Zr, Ce or la (2008) Top Catal, 49, pp. 46-58 | ||
| 504 | |a Aupretre, F., Descorme, C., Duprez, D., Casanave, D., Uzio, D.J., Ethanol steam reforming over Mg xNi 1-xAl 2O 3 spinel oxide-supported Rh catalysts (2005) J Catal, 233, pp. 464-477 | ||
| 504 | |a Iriondo, A., Barrio, V.L., Cambra, J.F., Arias, P.L., Guemez, M.B., Navarro, R.M., (2010) Glycerol Conversion into H 2 by Steam Reforming over Ni and PtNi Catalysts Supported on MgO Modified ã-Al 2O 3. Scientific Bases for the Preparation of Heterogeneous Catalysts, , Elsevier Amsterdam 449-452 | ||
| 504 | |a Koo, K.Y., Roh, H., Seo, Y.T., Seo, D.J., Yoon, W.L., Park, S.B., Coke study on MgO-promoted Ni/Al 2O 3 catalysts in combined H 2O and CO 2 reforming of methane for gas to liquid (GTL) process (2008) Appl Catal. A, 340, pp. 183-190 | ||
| 504 | |a Takehira, K., Shishido, T., Shouro, D., Murakami, K., Honda, M., Kawabata, T., Novel and effective surface enrichment of active species in Ni-loaded catalyst prepared from Mg-Al hydrotalcite-type anionic clay (2005) Appl Catal. A, 279, pp. 41-51 | ||
| 504 | |a Juan-Juan, J., Román Martínez, M.C., Illán-Gómez, M.J., Nickel catalyst activation in the carbon dioxide reforming of methane effect of pretreatments (2009) Appl Catal A, 355, pp. 27-32 | ||
| 506 | |2 openaire |e Política editorial | ||
| 520 | 3 | |a The aim of this work is to study the catalytic activity of Ni(10%) based catalysts supported over ã-Al 2O 3 modified with Mg (3%) for the steam reforming of glycerol. Catalysts have been prepared by incipient wetness impregnation method; analysing the effect of the calcination temperature of the modified support and the calcination temperature of the catalysts. Catalysts were characterized by temperature programmed reduction, (TPR), x-ray diffraction (DRX) and BET surface area. All catalysts were tested for this reaction in a fixed bed reactor. The best performance was achieved with the catalyst calcined at 500 °C being the optimum calcination temperature for the modified support of 900 °C This behaviour is ascribable to the formation of MgAl 2O 4 spinel which favours the dispersion of Ni°, responsible of the catalytic activity. © 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. |l eng | |
| 536 | |a Detalles de la financiación: Umweltbundesamt | ||
| 536 | |a Detalles de la financiación: Agencia Córdoba Ciencia | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas | ||
| 536 | |a Detalles de la financiación: We acknowledge the Fundación Peruilh, Agencia , CONICET , UBA for the financial support. | ||
| 593 | |a Laboratorio de Procesos Catalíticos, Departamento de Ing. Química, Ciudad Universitaria, 1428 C.A.B.A, Argentina | ||
| 593 | |a INQUIMAE, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria, 1428 C.A.B.A, Argentina | ||
| 690 | 1 | 0 | |a GLYCEROL |
| 690 | 1 | 0 | |a HYDROGEN |
| 690 | 1 | 0 | |a NI/MG/AL 2O 3 CATALYST |
| 690 | 1 | 0 | |a STEAM REFORMING |
| 690 | 1 | 0 | |a SYNGAS |
| 690 | 1 | 0 | |a BET SURFACE AREA |
| 690 | 1 | 0 | |a CALCINATION TEMPERATURE |
| 690 | 1 | 0 | |a FIXED BED REACTOR |
| 690 | 1 | 0 | |a INCIPIENT WETNESS IMPREGNATION METHOD |
| 690 | 1 | 0 | |a SYN-GAS |
| 690 | 1 | 0 | |a TEMPERATURE-PROGRAMMED REDUCTION |
| 690 | 1 | 0 | |a CALCINATION |
| 690 | 1 | 0 | |a CATALYST ACTIVITY |
| 690 | 1 | 0 | |a CHEMICAL REACTORS |
| 690 | 1 | 0 | |a GLYCEROL |
| 690 | 1 | 0 | |a HYDROGEN |
| 690 | 1 | 0 | |a STEAM REFORMING |
| 690 | 1 | 0 | |a SYNTHESIS GAS |
| 690 | 1 | 0 | |a X RAY DIFFRACTION |
| 690 | 1 | 0 | |a CATALYST SUPPORTS |
| 700 | 1 | |a Iannibelli, V. | |
| 700 | 1 | |a Jobbagy, M. | |
| 700 | 1 | |a Amadeo, Norma Elvira | |
| 773 | 0 | |d 2012 |g v. 37 |h pp. 14926-14930 |k n. 19 |p Int J Hydrogen Energy |x 03603199 |w (AR-BaUEN)CENRE-5264 |t International Journal of Hydrogen Energy | |
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