Synthesis of 17a-alkyl- and 17a-aryl-3β-acetoxy- and 3β-methoxy-17a-aza-d-homoandrost-5-en-17-one

A short and efficient preparation of 17a-methyl-, 17a-ethyl-, 17a-allyl-, and 17a-benzyl-3β-acetoxy-17a-aza-d-homoandrost-5-en-17-one, as well as 17a-methyl-, 17a-ethyl-, and 17a-allyl-3β-methoxy-17a-aza-s-homoandrost-5-en-17-one from the corresponding androsten-17-one derivatives is described. (Ste...

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Autor principal: Revelli, G.A
Otros Autores: Gros, E.G
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 1993
Acceso en línea:Registro en Scopus
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Registro en la Biblioteca Digital
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024 7 |2 scopus  |a 2-s2.0-0027324622 
024 7 |2 cas  |a 3-methoxy-17-aza-homoandrost-5-ene-17-one, 84300-23-2; Androstenols; Azasteroids 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a STEDA 
100 1 |a Revelli, G.A. 
245 1 0 |a Synthesis of 17a-alkyl- and 17a-aryl-3β-acetoxy- and 3β-methoxy-17a-aza-d-homoandrost-5-en-17-one 
260 |c 1993 
270 1 0 |m Gros, E.G. 
506 |2 openaire  |e Política editorial 
504 |a Doorenbos, Tamorria, Synthesis of some 4-azapregnanes (1965) J Pharm Sci, 54, pp. 1473-1476 
504 |a Chesnut, Durham, Brown, Mawdsley, Berlin, Antibacterial activity of 15-azasteroids alone and in combination with antibiotics (1976) Steroids, 27, pp. 525-541 
504 |a Chamberlin, Dehydroxymethyl derivatives of monensin (1974) Chem Abstr, 81, p. 135996x. , US Patent 3832358 
504 |a Michel, Hamill, Larsen, Williams, New azasteroidal antifungal antibiotics from Geotrichum flavobrunneum. II. Isolation and characterization (1975) J Antibiot (Tokyo), 28, pp. 102-105 
504 |a Gordee, Butler, New azasteroidal antifungal antibiotics from Geotrichum flavobrunneum. III. Biological activity (1975) J Antibiot (Tokyo), 28, pp. 112-117 
504 |a Boeck, Hoehn, Westhead, Wolter, Thomas, New azasteroidal antifungal antibiotics from Geotrichum flavobrunneum. I. Discovery and fermentation studies (1975) J Antibiot (Tokyo), 28, pp. 95-101 
504 |a Counsell, Klimstra, Nysted, Ranney, Hypocholesterolemic agents. V. Isomeric azacholesterols (1965) J Med Chem, 8, pp. 45-48 
504 |a Smith, Dupont, Influence of 20,25-diazocholesterol on serum lipoprotein lipids in mature rats (1967) Steroids, 9, pp. 85-96 
504 |a Singh, Bhardwaj, Ahuja, Paul, Steroids and related studies Part 44 17a-Methyl-3β-(N-pyrrolidinyl)-17a-aza-d-homo-5α-androstane bis(methiodide) (dihydrochaudonium iodide) and certain other analogs of chaudonium iodide (1979) Journal of the Chemical Society, Perkin Transactions 1, 1, pp. 305-307 
504 |a Bhardwaj, Kapoor, Shekar, Jindal, Singh, Steroids and related studies. Part 81. Potential azasteroidal neuromuscular blockers (1988) Indian J Chem, 27 B, pp. 209-212 
504 |a Rasmusson, Reynolds, Utne, Jobson, Primka, Berman, Brooks, Azasteroids as inhibitors of rat prostatic 5α-reductase (1984) J Med Chem, 27, pp. 1690-1701 
504 |a Weintraub, Blohm, Laughlin, Preparation of 20-(hydroxymethyl)-4-methyl-4-aza-2-oxa-5α-pregnan-3-one as an inhibitor of testosterone 5α-reductase (1985) J Med Chem, 28, pp. 831-833 
504 |a Rasmusson, Reynolds, Steinberg, Walton, Patel, Liang, Cascieri, Berman, Azasteroids structural activity relationships for inhibition of 5α-reductase and of androgen receptor binding (1986) J Med Chem, 29, pp. 2298-2315 
504 |a Stoka, Rivas, Segura, Rodriguez, Gros, Biological activity of synthetic juvenile hormone analogs (JHA) for Trypanosoma cruzi (1990) Z Naturforsch [c], 45 b, pp. 96-99. , (and previous papers cited therein) 
504 |a Kaufmann, Steroids. XVI. Beckmann rearrangement of 17-ketosteroids oximes (1951) J Am Chem Soc, 73, pp. 1779-1780 
504 |a Anliker, Müller, Wohlfahrt, Heusser, Über Steroid und Sexualhormone 168 Versuche zur einführung funktioneller Gruppen in die Stellung 18 des Steroid-gerüstes (1955) Helvetica Chimica Acta, 38, pp. 1404-1412 
504 |a Regan, Hayes, 17- and 17a-Aza-d-homosteroids (1956) J Am Chem Soc, 78, pp. 639-643 
504 |a Oka, Hara, Regiospecific Beckmann rearrangement of 3-oxo-4-ene steroids oximes (1978) J Org Chem, 43, pp. 3790-3791 
504 |a Dave, Stothers, Warnhoff, Resolution of conflicting migratory reports in ring expansion of 3-keto steroids (1980) Canadian Journal of Chemistry, 58, pp. 2666-2678 
504 |a Hendrickson, Bergeron, The protection and monoalkylation of amines (1970) Tetrahedron Letters, pp. 345-348 
504 |a Reuschling, Pietsch, Linkies, Eine einfache Methode zur N-alkylierung von β-Lactamen (1978) Tetrahedron Letters, pp. 615-618 
504 |a Johnstone, Rose, A rapid, simple and mild procedure for alkylation of phenols, alcohols, amides, and acids (1979) Tetrahedron, 35, pp. 2169-2173 
520 3 |a A short and efficient preparation of 17a-methyl-, 17a-ethyl-, 17a-allyl-, and 17a-benzyl-3β-acetoxy-17a-aza-d-homoandrost-5-en-17-one, as well as 17a-methyl-, 17a-ethyl-, and 17a-allyl-3β-methoxy-17a-aza-s-homoandrost-5-en-17-one from the corresponding androsten-17-one derivatives is described. (Steroids 58:181-184, 1993). © 1993.  |l eng 
536 |a Detalles de la financiación: Consejo Nacional de Rectores, T6cnicas 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: National Institute of Diabetes and Digestive and Kidney Diseases 
536 |a Detalles de la financiación: We thank Consejo Nacional de InvestigacioneCsi ent/-ficas y T6cnicas (CONICET) for partial financial support. We are also indebtedt o Unidad Microan~ilisiys M6todos Fisicos en Quimica Org~mica(U MYMFOR) (CONICET-FCEN) and Drs. D. Doller (Texas A & M University, College Station, Texas, USA) and L. Pannell (NIDDK, National Instituteso f Health, USA) for spectra.O ne of us (G.A.R.) thanks CONICET for a fellowship. 
593 |a Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Buenos Aires, Argentina 
690 1 0 |a 17A-AZA-D-HOMOANDROST-5-EN-17-ONE DERIVATIVES 
690 1 0 |a 13C NUCLEAR MAGNETIC RESONANCE SPECTRA 
690 1 0 |a 1H NUCLEAR MAGNETIC RESONANCE SPECTRA 
690 1 0 |a AZASTEROIDS 
690 1 0 |a SYNTHESIS 
690 1 0 |a 17A ALLYL 3BETA ACETOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A ALLYL 3BETA METHOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A BENZYL 3BETA ACETOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A ETHYL 3BETA ACETOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A ETHYL 3BETA METHOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A METHYL 3BETA ACETOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 17A METHYL 3BETA METHOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 3BETA ACETOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a 3BETA METHOXY 17A AZA D HOMOANDROST 5 EN 17 ONE 
690 1 0 |a AZASTEROID 
690 1 0 |a UNCLASSIFIED DRUG 
690 1 0 |a ARTICLE 
690 1 0 |a CARBON NUCLEAR MAGNETIC RESONANCE 
690 1 0 |a DRUG STRUCTURE 
690 1 0 |a DRUG SYNTHESIS 
690 1 0 |a MASS SPECTROMETRY 
690 1 0 |a PROTON NUCLEAR MAGNETIC RESONANCE 
690 1 0 |a ANDROSTENOLS 
690 1 0 |a AZASTEROIDS 
690 1 0 |a MAGNETIC RESONANCE SPECTROSCOPY 
690 1 0 |a MOLECULAR STRUCTURE 
690 1 0 |a SUPPORT, NON-U.S. GOV'T 
700 1 |a Gros, E.G. 
773 0 |d 1993  |g v. 58  |h pp. 181-184  |k n. 4  |p Steroids  |x 0039128X  |w (AR-BaUEN)CENRE-577  |t Steroids 
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