Solubility of solids in near-critical fluids III. CHI3 and CI4 in sulphur hexafluoride

The solubilities of CHI3(s) and CI4(s) in near-critical fluid SF6 have been spectrophotometrically determined. Due to the solubilities of the two solids in SF6, a new sampling and analytical procedure had to be developed to enable their measurement in the low solvent-density region, because they wer...

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Autor principal: Marceca, E.
Otros Autores: Fernández-Prini, R.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 1993
Acceso en línea:Registro en Scopus
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100 1 |a Marceca, E. 
245 1 0 |a Solubility of solids in near-critical fluids III. CHI3 and CI4 in sulphur hexafluoride 
260 |c 1993 
270 1 0 |m Fernández-Prini, R.; Departamento de Química Inorgánica, Analítica y Química Física and Instituto de Química Física de Materiales, Energía y Ambiente, 1428-Capital Federal, Argentina 
506 |2 openaire  |e Política editorial 
504 |a Fernández, D.P., Fernández-Prini, R., (1992) J. Chem. Thermodynamics, 24, p. 377 
504 |a Marceca, E., Fernández-Prini, R., (1993) J. Chem. Thermodynamics, 25, p. 237 
504 |a Rowlinson, J.S., Swinton, F.L., (1982) Liquids and Liquid Mixtures, p. 328. , Butterworths: London 
504 |a Lto, M., Huang, P.C., Kosower, E.M., (1961) Trans. Faraday Soc, 57, p. 1662 
504 |a Cole, W.A., Reuck, K.M., (1990) Int. J. Thermophys, 11, p. 189 
504 |a Gilgen, R., Kleinrahm, R., Wagner, W., (1992) J. Chem. Thermodynamics, 24, p. 953 
504 |a Biswas, S.N., Treppeniers, N.J., Hoogland, J.H.B., (1984) Physica, 126A, p. 384 
504 |a Fernández, Prini, R.;., Japas, M.L., (1992) J. Phys. Chem, 96, p. 5115 
504 |a Kumar, S.K., Johnston, K.P., (1988) J. Supercrit. Fluids, 1, p. 15 
520 3 |a The solubilities of CHI3(s) and CI4(s) in near-critical fluid SF6 have been spectrophotometrically determined. Due to the solubilities of the two solids in SF6, a new sampling and analytical procedure had to be developed to enable their measurement in the low solvent-density region, because they were below the detection limit of the previously developed spectrophotometric method. Isothermal solubility measurements were carried out under subcritical conditions in the dense liquid phase at temperature (302.20±0.01) K for CHI3 and (303.57±0.04) K for CI4, and under supercritical conditions at (322.76±0.03) K for CHI3 and (322.92±0.02) K for CI4; two isobaric runs were done for CHI3 at pressures of (3.818±0.003) MPa and (4.478±0.001) MPa. Solubilities depend strongly on p and T close to the thermodynamic state where the compressibility or thermal expansivity of the solvent pass, respectively, through a maximum. It is observed that CI4 is almost ten times less soluble than CHI3 in near-critical SF6. Moreover, the solubilities in SF6 are about ten times lower than in ethene. © 1993 Academic Press Ltd.  |l eng 
593 |a Departamento de Química Inorgánica, Analítica y Química Física and Instituto de Química Física de Materiales, Energía y Ambiente, 1428-Capital Federal, Argentina 
593 |a Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria Pabellón II, 1428-Capital Federal, Argentina 
700 1 |a Fernández-Prini, R. 
773 0 |d 1993  |g v. 25  |h pp. 719-728  |k n. 6  |p J Chem Thermodyn  |x 00219614  |w (AR-BaUEN)CENRE-575  |t The Journal of Chemical Thermodynamics 
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856 4 0 |u https://doi.org/10.1006/jcht.1993.1070  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_00219614_v25_n6_p719_Marceca  |y Handle 
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