Thermochemical kinetics of bromine nitrate, bromine nitrite, halogen hydroperoxides, dichlorine pentoxide, peroxycarboxylic acids, and diacyl peroxides

Heats of formation of BrONO2, BrONO, BrOOH, FOOH, FOOCl, CF3C(O)OOH, HC(O)OOH, CH3C(O)OOH, and [CH3C(O)O]2 are estimated from bond contributions taken from I. Phys. Chem., 100, 10150 (1996). They agree within ± 2 kcal/mol with recent experimental or ab initio data. The resulting BDE(O - O) = 36 kcal...

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Autor principal: Colussi, A.J
Otros Autores: Grela, M.A
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: John Wiley and Sons Inc. 1998
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100 1 |a Colussi, A.J. 
245 1 0 |a Thermochemical kinetics of bromine nitrate, bromine nitrite, halogen hydroperoxides, dichlorine pentoxide, peroxycarboxylic acids, and diacyl peroxides 
260 |b John Wiley and Sons Inc.  |c 1998 
270 1 0 |m Colussi, A.J.; Department of Physical Chemistry, Fac. of Exact and Natural Sciences, University of Buenos Aires, 1428-Buenos Aires, Argentina 
506 |2 openaire  |e Política editorial 
504 |a Grela, M.A., Colussi, A.J., (1996) J. Phys. Chem., 100, p. 10150 
504 |a Colussi, A.J., Grela, M.A., (1993) J. Phys. Chem., 97, p. 3775 
504 |a Orlando, J.J., Tyndall, G.S., (1996) J. Phys. Chem., 100, p. 19398 
504 |a Lee, T.J., (1996) J. Phys. Chem., 100, p. 19847 
504 |a Gillespie, R.J., Hargittai, I., (1991) The VSEPR Model of Molecular Geometry, , Allyn and Bacon, Boston 
504 |a Lee, T.J., (1996) Chem. Phys. Lett., 262, p. 559 
504 |a Hassanzadeh, P., Irikura, K.K., (1997) J. Phys. Chem., 101, p. 1580 
504 |a Ruscic, R., Berkowitz, J., (1994) J. Chem. Phys., 101, p. 7795 
504 |a Bogan, D.J., Thorn, R.P., Nesbitt, F.L., Stief, L.J., (1996) J. Phys. Chem., 100, p. 14383 
504 |a Grela, M.A., Colussi, A.J., to be submitted; Lee, T.J., Rice, J.E., Dateo, C.E., (1996) Mol. Phys., 89, p. 1359 
504 |a Francisco, J.S., (1993) J. Chem. Phys., 99, p. 10082 
504 |a Francisco, J.S., (1993) J. Chem. Phys., 98, p. 2198 
504 |a Francisco, J.S., (1996) J. Phys. Chem., 100, p. 10826 
504 |a Francisco, J.S., (1996) J. Chem. Phys., 105, p. 3338 
504 |a Jursic, B.S., (1997) J. Chem. Phys., 106, p. 2555 
504 |a Francisco, J.S., (1994) J. Phys. Chem., 98, p. 5650 
504 |a Colussi, A.J., Thermochemistry of Free Radicals (1988) Chemical Kinetics of Small Organic Radicals, 1, p. 25. , Z. B. Alfassi, Ed., CRC Press, Boca Raton 
504 |a (1994) NIST Standard Reference Database 25, Version 2.02, , National Bureau of Standards and Technology, Gaithersburg, Maryland 
504 |a Cohen, N., Benson, S.W., The Thermochemistry of Peroxides, Polyoxides and Their Free Radicals, , in press 
504 |a Bach, R.D., Ayala, P.Y., Schlegel, H.B., (1996) J. Am. Chem. Soc., 118, p. 12758 
504 |a Richardson, W.H., O'Neal, H.E., (1972) Chemical Kinetics, 5, pp. 486-487. , C. H. Bamford, C. F. H. Tipper, Elsevier, Amsterdam, and references therein 
504 |a Shine, H.J., Huffman, D.M., (1996) J. Am. Chem. Soc., 83, p. 2782 
504 |a note; Stull, D.R., Westrum, E.F., Sinke, G.C., (1969) The Chemical Thermodynamics of Organic Compounds, , Wiley, New York 
504 |a Cohen, N., Benson, S.W., (1993) Chem. Rev., 93, p. 2419 
504 |a Mauldin III, R.L., Burkholder, J.B., Ravishankara, A.R., (1997) Int. J. Chem. Kinet., 29, p. 139 
504 |a Colussi, A.J., (1990) J. Phys. Chem., 94, p. 8922 
504 |a Colussi, A.J., Sander, S.P., Friedl, R.R., (1992) J. Phys. Chem., 96, p. 4442 
504 |a While molecular reactivity is controlled by the properties of HOMO-LUMO frontier orbitals, bonding largely depends on localized valence interactions [29]; Selmi, M., Tomasi, J., J. Phys. Chem., 99, p. 5894 
504 |a Suidan, L., Badenhoop, J.K., Glendening, E.D., Weinhold, F., (1995) J. Chem. Educ., 72, p. 583 
520 3 |a Heats of formation of BrONO2, BrONO, BrOOH, FOOH, FOOCl, CF3C(O)OOH, HC(O)OOH, CH3C(O)OOH, and [CH3C(O)O]2 are estimated from bond contributions taken from I. Phys. Chem., 100, 10150 (1996). They agree within ± 2 kcal/mol with recent experimental or ab initio data. The resulting BDE(O - O) = 36 kcal/mol value in diacetyl peroxide requires the concerted assistance of exothermic C - C(O) weakening in the transition state of its decomposition into free radicals, It also implies the existence of a previously unrecognized 12 kcal/ mol nonbonded repulsion in acyl anhydrides, The formation of chloryl chlorate with ΔH1(O2ClOClO2) = 50 kcal/mol, a marginally stable species toward dissociation into (ClO3 + OClO), may account for observations made in the [O(3P) + OClO] system at low temperatures. © 1998 John Wiley & Sons, Inc.  |l eng 
593 |a Department of Physical Chemistry, Fac. of Exact and Natural Sciences, University of Buenos Aires, 1428-Buenos Aires, Argentina 
593 |a Department of Chemistry, University of Mar del Plata, P.O. Box 422, 7600-Mar del Plata, Argentina 
690 1 0 |a BROMINE COMPOUNDS 
690 1 0 |a CARBOXYLIC ACIDS 
690 1 0 |a DECOMPOSITION 
690 1 0 |a DISSOCIATION 
690 1 0 |a FREE RADICALS 
690 1 0 |a HALOGEN COMPOUNDS 
690 1 0 |a PEROXIDES 
690 1 0 |a CHEMICAL BONDS 
690 1 0 |a CHLORINE COMPOUNDS 
690 1 0 |a ELECTRON TRANSITIONS 
690 1 0 |a BROMINE NITRATE 
690 1 0 |a BROMINE NITRITE 
690 1 0 |a DIACYL PEROXIDES 
690 1 0 |a HALOGEN HYDROPEROXIDES 
690 1 0 |a PEROXYCARBOXYLIC ACIDS 
690 1 0 |a THERMOCHEMICAL KINETICS 
690 1 0 |a DICHLORINE PENTOXIDE 
690 1 0 |a THERMOCHEMISTRY 
690 1 0 |a REACTION KINETICS 
700 1 |a Grela, M.A. 
773 0 |d John Wiley and Sons Inc., 1998  |g v. 30  |h pp. 41-45  |k n. 1  |p Int J Chem Kinet  |x 05388066  |t International Journal of Chemical Kinetics 
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