An ATR-FTIR study of glyphosate and its Fe(III) complex in aqueous solution

An AIR-FTIR study of the vibrational spectrum of glyphosate (N- phosphonomethylglycine) in aqueous solution 1 M in NaCl is reported. Band assignments are given in the 1800-850 cm-1 range based on the analysis of the spectral changes from low to high pH values (2-11). Potentiometric titrations of gly...

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Autor principal: Barja, B.C
Otros Autores: Dos Santos Afonso, M.
Formato: Acta de conferencia Capítulo de libro
Lenguaje:Inglés
Publicado: ACS 1998
Acceso en línea:Registro en Scopus
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024 7 |2 scopus  |a 2-s2.0-0032212352 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a ESTHA 
100 1 |a Barja, B.C. 
245 1 3 |a An ATR-FTIR study of glyphosate and its Fe(III) complex in aqueous solution 
260 |b ACS  |c 1998 
270 1 0 |m Dos Santos Afonso, M.; Inquimae Depto. Quimica Inorganica, Analitica y Quimica Fisica, Universidad de Buenos Aires, Ciudad Universitaria, 1428 Buenos Aires, Argentina; email: dosantos@q3.fcen.uba.ar 
506 |2 openaire  |e Política editorial 
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504 |a Nakamoto, K., (1986) Infrared and Raman Spectra of Inorganic and Coordination Compounds; 4th Ed.; J. Wiley. New York 
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504 |a Bellamy, L.J., (1960) Tlie Infrared Spectra of Complex Molecules; J. Wiley: New York 
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520 3 |a An AIR-FTIR study of the vibrational spectrum of glyphosate (N- phosphonomethylglycine) in aqueous solution 1 M in NaCl is reported. Band assignments are given in the 1800-850 cm-1 range based on the analysis of the spectral changes from low to high pH values (2-11). Potentiometric titrations of glyphosate are performed at 0.1, 0.5, and 1 M ionic strengths in NaCl and the pK(a2), PK(a3), and pK(a4) values determined. A chemometric analysis of the spectral data has been carried out to support the assignments and reproduce the pKa values. In addition, the ATR-FTIR spectrum of the 1:1 Fe(III)/glyphosate complex in aqUeOuS solution is analyzed by comparison with that of the free ligand. An ATR-FTIR study of the vibrational spectrum of glyphosate (N-phosphonomethylglycine) in aqueous solution 1 M in NaCl is reported. Band assignments are given in the 1800-850 cm-1 range based on the analysis of the spectral changes from low to high pH values (2-11). Potentiometric titrations of glyphosate are performed at 0.1, 0.5, and 1 M ionic strengths in NaCl and the pKa2, pKa3, and pKa4 values determined. A chemometric analysis of the spectral data has been carried out to support the assignments and reproduce the pKa values. In addition, the ATR-FTIR spectrum of the 1:1 Fe(III)/glyphosate complex in aqueous solution is analyzed by comparison with that of the free ligand.  |l eng 
593 |a Inquimae Departamento de Quimica Inorgánica, Analítica y Química Física, Universidad de Buenos Aires, 1428, Buenos Aires, Argentina 
690 1 0 |a FOURIER TRANSFORM INFRARED SPECTROSCOPY 
690 1 0 |a HERBICIDES 
690 1 0 |a IONIC STRENGTH 
690 1 0 |a IRON 
690 1 0 |a PH EFFECTS 
690 1 0 |a SODIUM CHLORIDE 
690 1 0 |a SOLUTIONS 
690 1 0 |a TITRATION 
690 1 0 |a CHEMOMETRIC ANALYSIS 
690 1 0 |a GLYPHOSATE 
690 1 0 |a WATER POLLUTION 
690 1 0 |a GLYPHOSATE 
690 1 0 |a IRON COMPLEX 
690 1 0 |a AQUEOUS SOLUTION 
690 1 0 |a ARTICLE 
690 1 0 |a CHEMICAL ANALYSIS 
690 1 0 |a FOURIER TRANSFORMATION 
690 1 0 |a INFRARED SPECTROMETRY 
690 1 0 |a WATER POLLUTANT 
690 1 0 |a WATER POLLUTION 
700 1 |a Dos Santos Afonso, M. 
711 2 |c Washington, DC, United States 
773 0 |d ACS, 1998  |g v. 32  |h pp. 3331-3335  |k n. 21  |p Environ. Sci. Technol.  |x 0013936X  |w (AR-BaUEN)CENRE-14  |t Environmental Science and Technology 
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856 4 0 |u https://doi.org/10.1021/es9800380  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_0013936X_v32_n21_p3331_Barja  |y Handle 
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