Electrochemical behavior of Sn-Zn alloys with different grain structures in chloride-containing solutions

In the present research the electrochemical behavior of the Sn-Zn alloys (Sn-1. wt.%Zn, Sn-4. wt.%Zn and 8.9. wt.%Zn) in 3% NaCl solution is analyzed using potentiodynamic cyclic polarization measurements and Electrochemical Impedance Spectroscopy (EIS) technique. Specimens were longitudinally solid...

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Autor principal: Méndez, Claudia Marcela
Otros Autores: Scheiber, Verónica Liliana, Rozicki, Roberto Samuel, Kociubczyk, Alex Iván, Ares, Alicia Esther
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Elsevier B.V. 2016
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Acceso en línea:Registro en Scopus
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100 1 |a Méndez, Claudia Marcela 
245 1 0 |a Electrochemical behavior of Sn-Zn alloys with different grain structures in chloride-containing solutions 
260 |b Elsevier B.V.  |c 2016 
270 1 0 |m Ares, A.E.email: aares@fceqyn.unam.edu.ar 
506 |2 openaire  |e Política editorial 
520 3 |a In the present research the electrochemical behavior of the Sn-Zn alloys (Sn-1. wt.%Zn, Sn-4. wt.%Zn and 8.9. wt.%Zn) in 3% NaCl solution is analyzed using potentiodynamic cyclic polarization measurements and Electrochemical Impedance Spectroscopy (EIS) technique. Specimens were longitudinally solidified with simultaneous heat extraction in two opposite directions. Working electrodes were constructed using longitudinal and cross sections of the specimens with both types of structure: columnar and equiaxed.Results obtained from the polarization curves indicated that the two types of grain structures of Sn-Zn alloys (Sn-1. wt.%Zn, Sn-4. wt.%Zn and Sn-8.9. wt.%Zn) corresponding to longitudinal section present a pseudo passive zone. In the case of specimens from cross sections of the samples, the columnar and equiaxed zones of Sn-8.9. wt.%Zn are the only ones that do not have this pseudo passive region. In addition, the interdendritic zone of alloys is susceptible to corrosion by dealloying because this phase is zinc-rich. This type of corrosion also occurs in the zinc rich lamellar structure present in the eutectic. The percentage of zinc in the alloy increases with increasing susceptibility to pitting corrosion. The EIS values obtained revealed that the susceptibility to corrosion increases with increasing zinc content in alloys, for both the columnar and equiaxed zones. In addition, the columnar zones of Sn-4. wt.%Zn and Sn-8.9. wt.%Zn specimens are more resistant to corrosion than the equiaxed grain specimens. However, the equiaxed zone of Sn-1. wt.%Zn alloy is less susceptible to corrosion than the columnar zone. After adjustment by equivalent circuits it is revealed that the equiaxed zone of Sn-8.9. wt.%Zn alloy has a second porous layer composed of corrosion products on the electrode surface. © 2016 The Authors.  |l eng 
536 |a Article in Press 
593 |a Comité Ejecutivo de Desarrollo e Innovación Tecnológica (CEDIT), 3300 Posadas, Misiones, Argentina 
593 |a Instituto de Materiales de Misiones-IMAM (CONICET-UNaM), 3300 Posadas, Misiones, Argentina 
593 |a Programa de Materiales y Fisicoquímica (ProMyF), Facultad de Ciencias Exactas, Químicas y Naturales, Universidad Nacional de, Misiones, 3300 Posadas, Misiones, Argentina 
593 |a Carrera del Investigador Científico (CIC) at Consejo Nacional de Investigaciones Científicas y Tecnológicas (CONICET), Buenos Aires, Argentina 
650 1 7 |2 spines  |a CORROSION 
650 1 7 |2 spines  |a CORROSION 
690 1 0 |a EIS 
690 1 0 |a GRAIN STRUCTURES 
690 1 0 |a NACL 
690 1 0 |a SN-ZN ALLOYS 
690 1 0 |a BEHAVIORAL RESEARCH 
690 1 0 |a CRYSTAL MICROSTRUCTURE 
690 1 0 |a ELECTROCHEMICAL CORROSION 
690 1 0 |a ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY 
690 1 0 |a ELECTRODES 
690 1 0 |a EQUIVALENT CIRCUITS 
690 1 0 |a GRAIN SIZE AND SHAPE 
690 1 0 |a PITTING 
690 1 0 |a POLARIZATION 
690 1 0 |a TIN 
690 1 0 |a ZINC 
690 1 0 |a ZINC ALLOYS 
690 1 0 |a CORROSION PRODUCTS 
690 1 0 |a ELECTROCHEMICAL BEHAVIORS 
690 1 0 |a INTERDENDRITIC ZONES 
690 1 0 |a LONGITUDINAL SECTION 
690 1 0 |a NACL 
690 1 0 |a POLARIZATION CURVES 
690 1 0 |a POTENTIODYNAMIC CYCLIC POLARIZATIONS 
690 1 0 |a ZN ALLOYS 
690 1 0 |a TIN ALLOYS 
700 1 |a Scheiber, Verónica Liliana 
700 1 |a Rozicki, Roberto Samuel 
700 1 |a Kociubczyk, Alex Iván 
700 1 |a Ares, Alicia Esther 
773 0 |d Elsevier B.V., 2016  |x 18785352  |t Arab. J. Chem. 
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