Vapor phase hydrogenolysis of glycerol to 1,2-propanediol at atmospheric pressure over copper catalysts supported on mesoporous alumina
The present work explores the hydrogenolysis of glycerol to produce 1,2-propanediol in vapor phase at atmospheric pressure over copper catalysts supported on mesoporous alumina. Catalysts were prepared by alumina impregnation varying CuO loading between 3 wt% and 30 wt%. The textural and structural...
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| Formato: | Capítulo de libro |
| Lenguaje: | Inglés |
| Publicado: |
Elsevier B.V.
2017
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
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| LEADER | 08942caa a22011417a 4500 | ||
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| 001 | PAPER-15275 | ||
| 003 | AR-BaUEN | ||
| 005 | 20240927142613.0 | ||
| 008 | 190410s2017 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-85020388857 | |
| 030 | |a CATTE | ||
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Dieuzeide, M.L. | |
| 245 | 1 | 0 | |a Vapor phase hydrogenolysis of glycerol to 1,2-propanediol at atmospheric pressure over copper catalysts supported on mesoporous alumina |
| 260 | |b Elsevier B.V. |c 2017 | ||
| 270 | 1 | 0 | |m Amadeo, N.; ITHES (UBA-CONICET), Laboratorio de Procesos Catalíticos, Departamento de Ingeniería Química, Facultad de Ingeniería, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón de Industrias 1428, Ciudad Autónoma de Buenos AiresArgentina; email: norma@di.fcen.uba.ar |
| 504 | |a Katryniok, B., Paul, S., Dumeignil, F., (2013) ACS Catal., 3, pp. 1819-1834 | ||
| 504 | |a http://www.energia.gob.ar/contenidos/verpagina.php?idpagina=4008; Pagliaro, M., (2007) Angew. Chem. Int. Ed., 46, pp. 4434-4440 | ||
| 504 | |a Sun, D., Yamada, Y., Sato, S., Ueda, W., (2016) Appl. Catal. B: Environ., 193, pp. 75-92 | ||
| 504 | |a Chaminand, J., (2004) Green Chem., 6, pp. 359-361 | ||
| 504 | |a Dasari, M.A., Kiatsimkul, P., Sutterlin, W., Suppes, G., (2005) Appl. Catal. A: Gen., 281, pp. 225-231 | ||
| 504 | |a Kusunoki, Y., (2005) Catal. Commun., 6, pp. 645-649 | ||
| 504 | |a Sato, S., Akiyama, M., Takahashi, R., Hara, T., Iniu, K., Yokota, M., (2008) Appl. Catal. A: Gen., 347, pp. 186-191 | ||
| 504 | |a Vasiliadou, E.S., Lemonidou, A.A., (2011) Appl. Catal. A: Gen., 396, pp. 177-185 | ||
| 504 | |a Bienholz, A., (2011) Appl. Catal. A: Gen., 391, pp. 153-157 | ||
| 504 | |a Montassier, C., (1988) Studies Surf. Sci. Catal., 41, pp. 165-170 | ||
| 504 | |a Montassier, C., (1995) Appl. Catal. A: Gen., 121, pp. 231-244 | ||
| 504 | |a Huang, L., (2008) J. Chem. Technol. Biotechnol., 83, pp. 1670-1675 | ||
| 504 | |a Sato, S., Akiyama, M., Inui, K., Yokota, M., (2009) Chem. Lett., 38, pp. 560-569 | ||
| 504 | |a Akiyama, M., Sato, S., Takahashi, R., Inui, K., Yokota, M., (2009) Appl. Catal. A: Gen., 371, pp. 60-66 | ||
| 504 | |a Yuan, Z., Wang, J., Wang, L., Xie, W., Chen, P., Hou, Z., Zheng, X., (2010) Biores. Technol., 101, pp. 7088-7092 | ||
| 504 | |a Wang, Y., Zhou, J., Guo, X., (2015) RSC Adv., 5, pp. 74611-74628 | ||
| 504 | |a Guo, L., Zhou, J., Mao, J., Guo, X., Zhang, S., (2009) Appl. Catal. A: Gen., 367, pp. 93-98 | ||
| 504 | |a Gandarias, I., Arias, P.L., Requies, J., Guemez, M.B., Fierro, J.L.G., (2010) Appl. Catal. B: Environ., 97, pp. 248-256 | ||
| 504 | |a Feng, J., Xiang, W., Xu, B., Jiang, W., Wang, J., Chen, H., (2014) Catal. Commun., 46, pp. 98-102 | ||
| 504 | |a Chiu, C., Tekeei, A., Ronco, J., Banks, M., Suppes, G., (2008) Ind. Chem. Eng. Res., 47, pp. 6878-6884 | ||
| 504 | |a Chiu, C., Tekeei, A., Sutterlin, W., Ronco, J., Suppes, G., (2008) AIChE J., 54, pp. 2456-2463 | ||
| 504 | |a Vila, F., Lopez Granados, M., Ojeda, M., Fierro, J.L.G., Mariscal, R., (2012) Catal. Today, 187, pp. 122-128 | ||
| 504 | |a Sun, D., Yamada, Y., Sato, S., (2014) Appl. Catal. A: Gen., 475, pp. 63-68 | ||
| 504 | |a Dieuzeide, M.L., Jobbagy, M., Amadeo, N., (2016) Ind. Eng. Chem. Res., 55, pp. 2527-2533 | ||
| 504 | |a Zhu, S., Gao, X., Zhu, Y., Zhu, Y., Zheng, H., Li, Y., (2013) J. Catal., 303, pp. 70-79 | ||
| 504 | |a Vasiliadou, E.S., Eggenhuisen, T.M., Munnik, P., de Jongh, P.E., de Jong, K.P., Lemonidou, A.A., (2014) Appl. Catal. B: Environ., 145, pp. 108-119 | ||
| 504 | |a Feng, Y., (2011) Chem. Eng. J., 168, pp. 403-412 | ||
| 504 | |a Balaraju, M., Rekha, V., Sai Prasad, P.S., Prasad, R.B.N., Lingaiah, N., (2008) Catal. Lett, 126, pp. 119-124 | ||
| 504 | |a Yuan, Q., Ying, A.X., Luo, C., Sun, L.D., Zhang, Y.W., Duan, W.T., Liu, H.C., Yan, C.H., (2008) J. Am. Chem. Soc, 130, pp. 3465-3472 | ||
| 504 | |a Morris, S.M., Fulvio, P.F., Jaroniec, M., (2008) J. Am. Chem. Soc., 130, pp. 15210-15216 | ||
| 504 | |a Yuan, Q., Duan, H.H., Li, L.L., Li, Z.X., Duan, W.T., Zhang, L.S., Song, W.G., Yan, C.H., (2010) Adv. Mater., 22, pp. 1475-1478 | ||
| 504 | |a Cai, W.Q., Yu, J.G., Anand, C., Vinu, A., Jaroniec, M., (2011) Chem. Mater., 23, pp. 1147-1157 | ||
| 504 | |a Jiang, H., Bongard, H., Schmidt, W., Schüth, F., (2012) Microporous Mesoporous Mater., 164, pp. 3-8 | ||
| 504 | |a Patel, A., Shukla, P., Chen, J., Rufford, T.E., Wang, S., Rudolph, V., Zhu, Z., (2015) Chem. Eng. Res. Des., 101, pp. 27-43 | ||
| 504 | |a Ham, H., Kim, J., Cho, S.J., Choi, J.H., Moon, D.J., Bae, J.W., (2016) ACS Catal., 6, pp. 5629-5640 | ||
| 504 | |a Sato, S., Takahashi, R., Sodesawa, T., Yuma, K., Obata, Y., (2000) J. Catal., 196, pp. 195-199 | ||
| 504 | |a Gervasini, A., Bennici, S., (2005) Appl. Catal. A: Gen., 281, pp. 199-205 | ||
| 504 | |a Kruk, M., Jaroniec, M., (2001) Chem. Mater., 13, pp. 3169-3183 | ||
| 504 | |a Valange, S., Derouault, A., Barrault, J., Gabelica, Z., (2005) J. Mol. Catal. A: Chem., 228, pp. 255-266 | ||
| 504 | |a Dow, W., Wang, Y., Huang, T., (2000) Appl. Catal. A: Gen., 190, pp. 25-34 | ||
| 504 | |a Kim, J.Y., Rodriguez, J.A., Hanson, J.C., Frenkel, A.I., Lee, P.L., (2003) J. Am. Chem. Soc., 125, pp. 10684-10692 | ||
| 506 | |2 openaire |e Política editorial | ||
| 520 | 3 | |a The present work explores the hydrogenolysis of glycerol to produce 1,2-propanediol in vapor phase at atmospheric pressure over copper catalysts supported on mesoporous alumina. Catalysts were prepared by alumina impregnation varying CuO loading between 3 wt% and 30 wt%. The textural and structural characteristics of the catalysts were determined by N2 sorptometry (BET), powder X-ray diffraction (PXRD), temperature programmed reduction (TPR) and N2O chemisorption (copper metallic area). The characterization showed that all catalysts present textural properties characteristic of mesoporous solids, such as the adsorption isotherms which are type IV. Based both on characterization and activity results, it was possible to conclude that the yield to 1,2-propanediol presented a non-monotonic dependence on total copper metallic area. In addition, it was proved that 1,2-propanediol production is associated with the presence of highly dispersed CuO phase in the solids. Promising results were obtained with CuO(15)Al catalysts, taking into account that the performance can be improved by increasing residence time. © 2017 Elsevier B.V. |l eng | |
| 536 | |a Detalles de la financiación: Universidad de Buenos Aires | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP 0436 2012 | ||
| 536 | |a Detalles de la financiación: Authors would like to acknowledge UBA (UBACYT 2014-2017 398BA) and CONICET (PIP 0436 2012) for the financial support. | ||
| 593 | |a ITHES (UBA-CONICET), Laboratorio de Procesos Catalíticos, Departamento de Ingeniería Química, Facultad de Ingeniería, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón de Industrias, 1428 Ciudad Autónoma de Buenos Aires, Argentina | ||
| 593 | |a INQUIMAE (UBA-CONICET), Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria, 1428 Ciudad Autónoma de Buenos Aires, Argentina | ||
| 690 | 1 | 0 | |a 1,2-PROPANEDIOL |
| 690 | 1 | 0 | |a CUO CATALYSTS |
| 690 | 1 | 0 | |a GLYCEROL |
| 690 | 1 | 0 | |a HYDROGENOLYSIS |
| 690 | 1 | 0 | |a MESOPOROUS ALUMINA. |
| 690 | 1 | 0 | |a ALUMINA |
| 690 | 1 | 0 | |a ATMOSPHERIC PRESSURE |
| 690 | 1 | 0 | |a CATALYSTS |
| 690 | 1 | 0 | |a COPPER |
| 690 | 1 | 0 | |a COPPER OXIDES |
| 690 | 1 | 0 | |a GLYCEROL |
| 690 | 1 | 0 | |a HYDROGENOLYSIS |
| 690 | 1 | 0 | |a HYDROLYSIS |
| 690 | 1 | 0 | |a MESOPOROUS MATERIALS |
| 690 | 1 | 0 | |a X RAY DIFFRACTION |
| 690 | 1 | 0 | |a 1 ,2-PROPANEDIOL |
| 690 | 1 | 0 | |a CUO CATALYST |
| 690 | 1 | 0 | |a MESOPOROUS ALUMINA |
| 690 | 1 | 0 | |a NON-MONOTONIC DEPENDENCE |
| 690 | 1 | 0 | |a POWDER X-RAY DIFFRACTION (PXRD) |
| 690 | 1 | 0 | |a STRUCTURAL CHARACTERISTICS |
| 690 | 1 | 0 | |a TEMPERATURE-PROGRAMMED REDUCTION |
| 690 | 1 | 0 | |a TEXTURAL PROPERTIES |
| 690 | 1 | 0 | |a CATALYST SUPPORTS |
| 700 | 1 | |a de Urtiaga, R. | |
| 700 | 1 | |a Jobbagy, M. | |
| 700 | 1 | |a Amadeo, Norma Elvira | |
| 773 | 0 | |d Elsevier B.V., 2017 |g v. 296 |h pp. 19-25 |p Catal Today |x 09205861 |w (AR-BaUEN)CENRE-4117 |t Catalysis Today | |
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