Slow-release formulations of the herbicide picloram by using Fe–Al pillared montmorillonite
Slow-release formulations of the herbicide picloram (PCM, 4-amino-3,5,6-trichloropyridine-2-carboxylic acid) were designed based on its adsorption on pillared clays (pillared clays (PILCs)) for reducing the water-polluting risk derived from its use in conventional formulations. Fe–Al PILCs were synt...
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Springer Verlag
2017
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| LEADER | 17675caa a22013577a 4500 | ||
|---|---|---|---|
| 001 | PAPER-15092 | ||
| 003 | AR-BaUEN | ||
| 005 | 20230518204545.0 | ||
| 008 | 190410s2017 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-85014678911 | |
| 024 | 7 | |2 cas |a aluminum silicate, 12183-80-1, 1302-93-8, 1318-74-7, 1335-30-4, 61027-90-5; bentonite, 1302-78-9; picloram, 1918-02-1; Aluminum Silicates; Bentonite; clay; Herbicides; Picloram | |
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 030 | |a ESPLE | ||
| 100 | 1 | |a Marco-Brown, J.L. | |
| 245 | 1 | 0 | |a Slow-release formulations of the herbicide picloram by using Fe–Al pillared montmorillonite |
| 260 | |b Springer Verlag |c 2017 | ||
| 270 | 1 | 0 | |m Marco-Brown, J.L.; Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón II, Argentina; email: josemarcobrown@gmail.com |
| 506 | |2 openaire |e Política editorial | ||
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| 520 | 3 | |a Slow-release formulations of the herbicide picloram (PCM, 4-amino-3,5,6-trichloropyridine-2-carboxylic acid) were designed based on its adsorption on pillared clays (pillared clays (PILCs)) for reducing the water-polluting risk derived from its use in conventional formulations. Fe–Al PILCs were synthesized by the reaction of Na+-montmorillonite (SWy-2) with base-hydrolyzed solutions of Fe and Al. The Fe/(Fe + Al) ratios used were 0.15 and 0.50. The PCM adsorption isotherms on Fe–Al PILCs were well fitted to Langmuir and Freundlich models. The PCM adsorption capacity depended on the Fe content in the PILCs. Slow-release formulations were prepared by enhanced adsorption of the herbicide from PCM-cyclodextrin (CD) complexes in solution. CDs were able to enhance up to 2.5-fold the solubility of PCM by the formation of inclusion complexes where the ring moiety of the herbicide was partially trapped within the CD cavity. Competitive adsorption of anions such as sulfate, phosphate, and chloride as well as the FTIR analysis of PCM-PILC complexes provided evidence of formation of inner sphere complexes of PCM-CD on Fe–Al PILCs. Release of the herbicide in a sandy soil was lower from Fe–Al PILC formulations relative to a PCM commercial formulation. © 2017, Springer-Verlag Berlin Heidelberg. |l eng | |
| 536 | |a Detalles de la financiación: Secretaria Nacional de Ciencia y Tecnología | ||
| 536 | |a Detalles de la financiación: Ministerio de la Producción, Ciencia y Tecnología | ||
| 536 | |a Detalles de la financiación: Ministerio de Educación y Cultura, CTM2013-42306-R | ||
| 536 | |a Detalles de la financiación: Universidad de Buenos Aires | ||
| 536 | |a Detalles de la financiación: European Social Fund, ESF | ||
| 536 | |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas | ||
| 536 | |a Detalles de la financiación: P12-RNM1897 | ||
| 536 | |a Detalles de la financiación: The authors acknowledge Universidad de Buenos Aires, Secretaria de Ciencia y T?cnica Projects, Ministerio de Ciencia y T?cnica, Agencia Nacional de Promoci?n Cient?fica y Tecnol?gica, MINCyT-ANPCyT-FONCyT, and Consejo Nacional de Investigaciones Cient?ficas y T?cnicas de la Rep?blica Argentina (CONICET) for financial support. J.L.M-B acknowledges CONICET fellowship. This research was also supported by the MEC Project CTM2013-42306-R and the Junta de Andaluc?a Project P12-RNM1897. Both projects received funding by the European Social Fund. The authors also acknowledge the Analytical Services of Seville University (CITIUS) for SEM-EDS measurements. | ||
| 593 | |a Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón II, Buenos Aires, C1428EHA, Argentina | ||
| 593 | |a Instituto de Química Física de los Materiales, Medio Ambiente y Energía de la Facultad de Ciencias Exactas y Naturales (INQUIMAE), CONICET-Universidad de Buenos Aires, Buenos Aires, Argentina | ||
| 593 | |a Instituto de Investigación e Ingeniería Ambiental (3iA), CONICET, Escuela de Ciencia y Tecnología, UNSAM, 25 de Mayo y Francia (1650), San Martín, Argentina | ||
| 593 | |a Institute of Natural Resources and Agrobiology (IRNAS-CSIC), Reina Mercedes 10. Apdo. 1052, Sevilla, 41080, Spain | ||
| 593 | |a Centro de Tecnología en Recursos Minerales y Cerámica (CETMIC), CONICET-CCT La Plata-CIC, Camino Centenario y 506 CC (49), M. B. Gonnet, B1897ZCA, Argentina | ||
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a FE–AL PILLARED MONTMORILLONITE |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a SLOW-RELEASE FORMULATIONS |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ANION |
| 690 | 1 | 0 | |a HERBICIDE |
| 690 | 1 | 0 | |a HYDROLYSIS |
| 690 | 1 | 0 | |a MONTMORILLONITE |
| 690 | 1 | 0 | |a PESTICIDE RESIDUE |
| 690 | 1 | 0 | |a SANDY SOIL |
| 690 | 1 | 0 | |a WATER POLLUTION |
| 690 | 1 | 0 | |a ALUMINUM SILICATE |
| 690 | 1 | 0 | |a BENTONITE |
| 690 | 1 | 0 | |a CLAY |
| 690 | 1 | 0 | |a HERBICIDE |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ALUMINUM SILICATES |
| 690 | 1 | 0 | |a BENTONITE |
| 690 | 1 | 0 | |a HERBICIDES |
| 690 | 1 | 0 | |a PICLORAM |
| 700 | 1 | |a Undabeytia, T. | |
| 700 | 1 | |a Torres Sánchez, R.M. | |
| 700 | 1 | |a dos Santos Afonso, M. | |
| 773 | 0 | |d Springer Verlag, 2017 |g v. 24 |h pp. 10410-10420 |k n. 11 |p Environ. Sci. Pollut. Res. |x 09441344 |t Environmental Science and Pollution Research | |
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