Insights into dimethyl sulfoxide decomposition in Li-O2 battery: Understanding carbon dioxide evolution

DMSO has been widely investigated as a potential electrolyte for the Li-air battery systems, however its stability has been a topic of debate in the research community. In this communication we have identified the side reaction products during the oxygen reduction reaction (ORR) and oxygen evolution...

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Autor principal: Mozhzhukhina, N.
Otros Autores: Marchini, F., Torres, W.R, Tesio, A.Y, Mendez De Leo, L.P, Williams, F.J, Calvo, E.J
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: Elsevier Inc. 2017
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100 1 |a Mozhzhukhina, N. 
245 1 0 |a Insights into dimethyl sulfoxide decomposition in Li-O2 battery: Understanding carbon dioxide evolution 
260 |b Elsevier Inc.  |c 2017 
270 1 0 |m Calvo, E.J.; Departamento de Química Inorgánica, Analítica y Química Física, INQUIMAE-CONICET, Facultad Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón 2, Argentina; email: calvo@qi.fcen.uba.ar 
506 |2 openaire  |e Política editorial 
504 |a Aurbach, D., McCloskey, B.D., Nazar, L.F., Bruce, P.G., Advances in understanding mechanisms underpinning lithium–air batteries (2016) Nat. Energy, 1, p. 16128 
504 |a Amine, K., Kanno, R., Tzeng, Y., Rechargeable lithium batteries and beyond: progress, challenges, and future directions (2014) MRS Bull., 39 (5), pp. 395-401 
504 |a Grande, L., Paillard, E., Hassoun, J., Park, J.B., Lee, Y.J., Sun, Y.K., Passerini, S., Scrosati, B., The lithium/air battery: still an emerging system or a practical reality? (2015) Adv. Mater., 27 (5), pp. 784-800 
504 |a Luntz, A.C., McCloskey, B.D., Nonaqueous Li-air batteries: a status report (2014) Chem. Rev., 114 (23), pp. 11721-11750 
504 |a McCloskey, B.D., Burke, C.M., Nichols, J.E., Renfrew, S.E., Mechanistic insights for the development of Li-O2 battery materials: addressing Li2O2 conductivity limitations and electrolyte and cathode instabilities (2015) Chem. Commun., 51 (64), pp. 12701-12715 
504 |a Trahan, M.J., Mukerjee, S., Plichta, E.J., Hendrickson, M.A., Abraham, K.M., Studies of Li-air cells utilizing dimethyl sulfoxide-based electrolyte (2012) J. Electrochem. Soc., 160 (2), pp. A259-A267 
504 |a Peng, Z., Freunberger, S.A., Chen, Y., Bruce, P.G., A reversible and higher-rate Li-O2 battery (2012) Science, 337 (6094), pp. 563-566 
504 |a Xu, W., Hu, J., Engelhard, M.H., Towne, S.A., Hardy, J.S., Xiao, J., Feng, J., Zhang, J.-G., The stability of organic solvents and carbon electrode in nonaqueous Li-O2 batteries (2012) J. Power Sources, 215, pp. 240-247 
504 |a Schroeder, M.A., Kumar, N., Pearse, A.J., Liu, C., Lee, S.B., Rubloff, G.W., Leung, K., Noked, M., DMSO-Li2O2 interface in the rechargeable Li-O2 battery cathode: theoretical and experimental perspectives on stability (2015) ACS Appl. Mater. Interfaces, 7 (21), pp. 11402-11411 
504 |a Marchini, F., Herrera, S., Torres, W., Tesio, A.Y., Williams, F.J., Calvo, E.J., Surface study of lithium-air battery oxygen cathodes in different solvent-electrolyte pairs (2015) Langmuir, 31 (33), pp. 9236-9245 
504 |a Marchini, F., Herrera, S.E., Calvo, E.J., Williams, F.J., Surface studies of lithium–oxygen redox reactions over HOPG (2016) Surf. Sci., 646, pp. 154-159 
504 |a Younesi, R., Norby, P., Vegge, T., A new look at the stability of dimethyl sulfoxide and acetonitrile in Li-O2 batteries (2014) ECS Electrochem. Lett., 3 (3), pp. A15-A18 
504 |a Kwabi, D.G., Batcho, T.P., Amanchukwu, C.V., Ortiz-Vitoriano, N., Hammond, P., Thompson, C.V., Shao-Horn, Y., Chemical instability of dimethyl sulfoxide in lithium-air batteries (2014) J. Phys. Chem. Lett., 5 (16), pp. 2850-2856 
504 |a Sharon, D., Afri, M., Noked, M., Garsuch, A., Frimer, A.A., Aurbach, D., Oxidation of dimethyl sulfoxide solutions by electrochemical reduction of oxygen (2013) J. Phys. Chem. Lett., 4 (18), pp. 3115-3119 
504 |a Mozhzhukhina, N., Méndez De Leo, L.P., Calvo, E.J., Infrared spectroscopy studies on stability of dimethyl sulfoxide for application in a Li–air battery (2013) J. Phys. Chem. C, 117 (36), pp. 18375-18380 
504 |a Calvo, E.J., Mozhzhukhina, N., A rotating ring disk electrode study of the oxygen reduction reaction in lithium containing non aqueous electrolyte (2013) Electrochem. Commun., 31, pp. 56-58 
504 |a Torres, W., Mozhzhukhina, N., Tesio, A.Y., Calvo, E.J., A rotating ring disk electrode study of the oxygen reduction reaction in lithium containing dimethyl sulfoxide electrolyte: role of superoxide (2014) J. Electrochem. Soc., 161 (14), pp. A2204-A2209 
504 |a Mozhzhukhina, N., Tesio, A.Y., De Leo, L.P.M., Calvo, E.J., In situ infrared spectroscopy study of PYR14TFSI ionic liquid stability for Li–O2 battery (2017) J. Electrochem. Soc., 164 (2), pp. A518-A523 
504 |a De Leo, L.P.M., De La Llave, E., Scherlis, D., Williams, F.J., Molecular and electronic structure of electroactive self-assembled monolayers (2013) J. Chem. Phys., 138 (11) 
520 3 |a DMSO has been widely investigated as a potential electrolyte for the Li-air battery systems, however its stability has been a topic of debate in the research community. In this communication we have identified the side reaction products during the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) on Au in dimethyl sulfoxide-based electrolyte for Li-air battery by a combination of in-situ analytical tools: EQCM, SNIFTIRS, DEMS and XPS, in particular the evolution of CO2 from the solvent decomposition. © 2017 Elsevier B.V.  |l eng 
536 |a Detalles de la financiación: Universidad de Buenos Aires 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PICT 2014V, 3654 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: Funding from UBA, CONICET and ANPCyT PICT 2014V No. 3654 are gratefully acknowledged. NM, FM, WRT have doctoral fellowships and A.Y.T a postdoctoral fellowship form CONICET which are gratefully acknowledged. 
593 |a Departamento de Química Inorgánica, Analítica y Química Física, INQUIMAE-CONICET, Facultad Ciencias Exactas y Naturales, Universidad de Buenos Aires, Ciudad Universitaria, Pabellón 2, Buenos Aires, C1428EHA, Argentina 
690 1 0 |a AIR 
690 1 0 |a BATTERY 
690 1 0 |a CO2 
690 1 0 |a DMSO 
690 1 0 |a LITHIUM 
690 1 0 |a OXYGEN 
690 1 0 |a AIR 
690 1 0 |a CARBON DIOXIDE 
690 1 0 |a DIMETHYL SULFOXIDE 
690 1 0 |a ELECTRIC BATTERIES 
690 1 0 |a ELECTROLYTES 
690 1 0 |a ELECTROLYTIC REDUCTION 
690 1 0 |a LITHIUM 
690 1 0 |a ORGANIC SOLVENTS 
690 1 0 |a OXYGEN 
690 1 0 |a BATTERY 
690 1 0 |a CARBON DIOXIDE EVOLUTION 
690 1 0 |a DMSO 
690 1 0 |a LI-AIR BATTERIES 
690 1 0 |a OXYGEN EVOLUTION REACTION 
690 1 0 |a OXYGEN REDUCTION REACTION 
690 1 0 |a RESEARCH COMMUNITIES 
690 1 0 |a SOLVENT DECOMPOSITIONS 
690 1 0 |a LITHIUM BATTERIES 
650 1 7 |2 spines  |a CARBON 
700 1 |a Marchini, F. 
700 1 |a Torres, W.R. 
700 1 |a Tesio, A.Y. 
700 1 |a Mendez De Leo, L.P. 
700 1 |a Williams, F.J. 
700 1 |a Calvo, E.J. 
773 0 |d Elsevier Inc., 2017  |g v. 80  |h pp. 16-19  |p Electrochem. Commun.  |x 13882481  |w (AR-BaUEN)CENRE-1729  |t Electrochemistry Communications 
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