New insights on the structure of the picloram-montmorillonite surface complexes
Hypothesis: The environmental mobility and bioavailability of Picloram (PCM) are determined by the amine and carboxylate chemical groups interaction with the soils mineral phases. Clay particles, such as montmorillonite (Mt), and the pH value of the media could play an important role in adsorption p...
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| Otros Autores: | , , , |
| Formato: | Capítulo de libro |
| Lenguaje: | Inglés |
| Publicado: |
Academic Press Inc.
2015
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
| Aporte de: | Registro referencial: Solicitar el recurso aquí |
| LEADER | 12608caa a22018257a 4500 | ||
|---|---|---|---|
| 001 | PAPER-13480 | ||
| 003 | AR-BaUEN | ||
| 005 | 20230518204350.0 | ||
| 008 | 190411s2015 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-84921033392 | |
| 024 | 7 | |2 cas |a montmorillonite, 1318-93-0, 61029-13-8; picloram, 1918-02-1; aluminum silicate, 12183-80-1, 1302-93-8, 1318-74-7, 1335-30-4, 61027-90-5; bentonite, 1302-78-9; Aluminum Silicates; Bentonite; clay; Herbicides; Picloram; Soil | |
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 030 | |a JCISA | ||
| 100 | 1 | |a Marco-Brown, J.L. | |
| 245 | 1 | 0 | |a New insights on the structure of the picloram-montmorillonite surface complexes |
| 260 | |b Academic Press Inc. |c 2015 | ||
| 270 | 1 | 0 | |m Dos Santos Afonso, M.; Departamento de Química Inorgánica, Analítica y Química Física e INQUIMAE, FCEN, UBA, Ciudad Universitaria, Pabellón II, Argentina |
| 506 | |2 openaire |e Política editorial | ||
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| 520 | 3 | |a Hypothesis: The environmental mobility and bioavailability of Picloram (PCM) are determined by the amine and carboxylate chemical groups interaction with the soils mineral phases. Clay particles, such as montmorillonite (Mt), and the pH value of the media could play an important role in adsorption processes. Thus, the study of the role of soil components other than organic matter deserves further investigation for a more accurate assessment of the risk of groundwater contamination. Experiments: Samples with PCM adsorbed on Mt dispersions were prepared at pH 3-9. Subsequently, the dispersions were separated, washed, centrifuged and stored at room temperature. Picloram (PCM) herbicide interaction with surface groups of montmorillonite (Mt) was studied using XRD, DTA, FTIR and XPS techniques. Findings: The entrance of PCM into the Mt basal space, in two different arrangements, perpendicular and planar, is proposed and the final arrangement depends on PCM concentration. The interaction of PCM with Mt surface sites through the nitrogen of the pyridine ring and carboxylic group of PCM, forming bidentate and bridge inner-sphere complexes was confirmed by FTIR and XPS analysis. The acidity constant of the PCM adsorbed on the Mt surface was calculated. © 2014 Elsevier Inc. |l eng | |
| 536 | |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica | ||
| 536 | |a Detalles de la financiación: BE/PA05-EXIII/001 | ||
| 536 | |a Detalles de la financiación: Universidad de Buenos Aires | ||
| 536 | |a Detalles de la financiación: Ministerio de la Producción, Ciencia y Tecnología | ||
| 536 | |a Detalles de la financiación: Secretaría de Ciencia y Técnica, Universidad de Buenos Aires, X043, PICT 23-32678, X067 | ||
| 536 | |a Detalles de la financiación: Fondo para la Investigación Científica y Tecnológica | ||
| 536 | |a Detalles de la financiación: The authors acknowledge the Universidad de Buenos Aires (UBA) and Ministerio de Ciencia y Tecnología, Agencia Nacional de Promoción Científica y Tecnológica, Fondo para la Investigación Científica y Tecnológica (MINCyT-ANPCyT-FONCyT) for financial support through UBACyT X043, X067, PICT 23-32678 and SECyT/FNRS BE/PA05-EXIII/001 grants. R.M.T.S is member of CONICET and J.L.M-B and M.A.T. acknowledge CONICET fellowships. The authors also are grateful to Michel I. Genet for his assistance with XPS interpretation. Appendix A | ||
| 593 | |a Departamento de Química Inorgánica, Analítica y Química Física e INQUIMAE, FCEN, UBA, Ciudad Universitaria, Pabellón II, Buenos Aires, C1428EHA, Argentina | ||
| 593 | |a Université Catholique de Louvain, Institute of Condensed Matter and Nanosciences (IMCN), Division Solids, Molecules and Reactivity (MOST), Croix du Sud 2/L7.05.17, Louvain-la-Neuve, B-1348, Belgium | ||
| 593 | |a CETMIC (Centro de Tecnología en Minerales y Cerámica), Camino Centenario y 506 CC (49), M. B. Gonnet, B1897ZCA, Argentina | ||
| 690 | 1 | 0 | |a CLAY MINERALS |
| 690 | 1 | 0 | |a MONTMORILLONITE |
| 690 | 1 | 0 | |a PICLORAM HERBICIDE |
| 690 | 1 | 0 | |a SURFACE COMPLEXES |
| 690 | 1 | 0 | |a BIOCHEMISTRY |
| 690 | 1 | 0 | |a CARBOXYLATION |
| 690 | 1 | 0 | |a CLAY MINERALS |
| 690 | 1 | 0 | |a DISPERSIONS |
| 690 | 1 | 0 | |a GROUNDWATER |
| 690 | 1 | 0 | |a GROUNDWATER POLLUTION |
| 690 | 1 | 0 | |a PYRIDINE |
| 690 | 1 | 0 | |a RISK ASSESSMENT |
| 690 | 1 | 0 | |a WEED CONTROL |
| 690 | 1 | 0 | |a X RAY PHOTOELECTRON SPECTROSCOPY |
| 690 | 1 | 0 | |a ADSORPTION PROCESS |
| 690 | 1 | 0 | |a ENVIRONMENTAL MOBILITY |
| 690 | 1 | 0 | |a GROUNDWATER CONTAMINATION |
| 690 | 1 | 0 | |a INNER SPHERE COMPLEXES |
| 690 | 1 | 0 | |a MONTMORILLONITE SURFACE |
| 690 | 1 | 0 | |a MONTMORILLONITES (MT) |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a SURFACE COMPLEX |
| 690 | 1 | 0 | |a HERBICIDES |
| 690 | 1 | 0 | |a GROUND WATER |
| 690 | 1 | 0 | |a MONTMORILLONITE |
| 690 | 1 | 0 | |a ORGANIC MATTER |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a ALUMINUM SILICATE |
| 690 | 1 | 0 | |a BENTONITE |
| 690 | 1 | 0 | |a CLAY |
| 690 | 1 | 0 | |a HERBICIDE |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a SOIL |
| 690 | 1 | 0 | |a ACID DISSOCIATION CONSTANT |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ARTICLE |
| 690 | 1 | 0 | |a CLAY |
| 690 | 1 | 0 | |a COMPLEX FORMATION |
| 690 | 1 | 0 | |a DESORPTION |
| 690 | 1 | 0 | |a DISPERSION |
| 690 | 1 | 0 | |a EQUILIBRIUM CONSTANT |
| 690 | 1 | 0 | |a POROSITY |
| 690 | 1 | 0 | |a PRIORITY JOURNAL |
| 690 | 1 | 0 | |a SOIL PROPERTY |
| 690 | 1 | 0 | |a THERMOGRAVIMETRY |
| 690 | 1 | 0 | |a WATER CONTAMINATION |
| 690 | 1 | 0 | |a X RAY DIFFRACTION |
| 690 | 1 | 0 | |a X RAY PHOTOELECTRON SPECTROSCOPY |
| 690 | 1 | 0 | |a CHEMISTRY |
| 690 | 1 | 0 | |a INFRARED SPECTROSCOPY |
| 690 | 1 | 0 | |a SOIL |
| 690 | 1 | 0 | |a SURFACE PROPERTY |
| 690 | 1 | 0 | |a ADSORPTION |
| 690 | 1 | 0 | |a ALUMINUM SILICATES |
| 690 | 1 | 0 | |a BENTONITE |
| 690 | 1 | 0 | |a HERBICIDES |
| 690 | 1 | 0 | |a PHOTOELECTRON SPECTROSCOPY |
| 690 | 1 | 0 | |a PICLORAM |
| 690 | 1 | 0 | |a SOIL |
| 690 | 1 | 0 | |a SPECTROSCOPY, FOURIER TRANSFORM INFRARED |
| 690 | 1 | 0 | |a SURFACE PROPERTIES |
| 690 | 1 | 0 | |a X-RAY DIFFRACTION |
| 650 | 1 | 7 | |2 spines |a PH |
| 700 | 1 | |a Trinelli, M.A. | |
| 700 | 1 | |a Gaigneaux, E.M. | |
| 700 | 1 | |a Torres Sánchez, R.M. | |
| 700 | 1 | |a Dos Santos Afonso, M. | |
| 773 | 0 | |d Academic Press Inc., 2015 |g v. 444 |h pp. 115-122 |p J. Colloid Interface Sci. |x 00219797 |w (AR-BaUEN)CENRE-15 |t Journal of Colloid and Interface Science | |
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