Salt Pumping by Voltage-Gated Nanochannels
This Letter investigates voltage-gated nanochannels, where both the potential applied to the conductive membrane containing the channel (membrane potential) and the potential difference between the solutions at both sides of the membrane (transmembrane potential) are independently controlled. The pr...
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| Formato: | Capítulo de libro |
| Lenguaje: | Inglés |
| Publicado: |
American Chemical Society
2015
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| Acceso en línea: | Registro en Scopus DOI Handle Registro en la Biblioteca Digital |
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| LEADER | 09999caa a22009977a 4500 | ||
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| 001 | PAPER-13312 | ||
| 003 | AR-BaUEN | ||
| 005 | 20230518204338.0 | ||
| 008 | 190411s2015 xx ||||fo|||| 00| 0 eng|d | ||
| 024 | 7 | |2 scopus |a 2-s2.0-84942017781 | |
| 040 | |a Scopus |b spa |c AR-BaUEN |d AR-BaUEN | ||
| 100 | 1 | |a Tagliazucchi, M. | |
| 245 | 1 | 0 | |a Salt Pumping by Voltage-Gated Nanochannels |
| 260 | |b American Chemical Society |c 2015 | ||
| 270 | 1 | 0 | |m Szleifer, I.; Department of Biomedical Engineering, Department of Chemistry and Chemistry of Life Processes Institute, Northwestern UniversityUnited States |
| 506 | |2 openaire |e Política editorial | ||
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| 520 | 3 | |a This Letter investigates voltage-gated nanochannels, where both the potential applied to the conductive membrane containing the channel (membrane potential) and the potential difference between the solutions at both sides of the membrane (transmembrane potential) are independently controlled. The predicted conductance characteristics of these fixed-potential channels dramatically differ from those of the widely studied fixed-charge nanochannels, in which the membrane is insulating and has a fixed surface charge density. The difference arises because the transmembrane potential induces an inhomogeneous charge distribution on the surface of fixed-potential nanochannels. This behavior, related to bipolar electrochemistry, has some interesting and unexpected consequences for ion transport. For example, continuously oscillating the transmembrane potential, while holding the membrane potential at the potential for which it has zero charge in equilibrium, creates fluxes of neutral salt (fluxes of anions and cations in the same direction and number) through the channel, which is an interesting phenomenon for desalination applications. © 2015 American Chemical Society. |l eng | |
| 536 | |a Detalles de la financiación: Basic Energy Sciences, BES, DE-SC0000989 | ||
| 536 | |a Detalles de la financiación: U.S. Department of Energy, DOE | ||
| 536 | |a Detalles de la financiación: Office of Science, SC | ||
| 593 | |a Department of Biomedical Engineering, Department of Chemistry and Chemistry of Life Processes Institute, Northwestern University, Evanston, IL 60208, United States | ||
| 593 | |a INQUIMAE-CONICET, Ciudad Universitaria, Pabellón 2, Ciudad Autónoma de Buenos Aires, C1428EHA, Argentina | ||
| 690 | 1 | 0 | |a BIPOLAR DIODE |
| 690 | 1 | 0 | |a BIPOLAR ELECTROCHEMISTRY |
| 690 | 1 | 0 | |a DESALINIZATION |
| 690 | 1 | 0 | |a ION CURRENT |
| 690 | 1 | 0 | |a MEMBRANE |
| 690 | 1 | 0 | |a NANOPORE |
| 690 | 1 | 0 | |a NERNST-PLANCK |
| 690 | 1 | 0 | |a BIOELECTRIC POTENTIALS |
| 690 | 1 | 0 | |a DESALINATION |
| 690 | 1 | 0 | |a ELECTROCHEMISTRY |
| 690 | 1 | 0 | |a IONS |
| 690 | 1 | 0 | |a NANOPORES |
| 690 | 1 | 0 | |a BIPOLAR DIODES |
| 690 | 1 | 0 | |a BIPOLAR ELECTROCHEMISTRIES |
| 690 | 1 | 0 | |a DESALINIZATION |
| 690 | 1 | 0 | |a ION CURRENTS |
| 690 | 1 | 0 | |a NERNST-PLANCK |
| 690 | 1 | 0 | |a MEMBRANES |
| 700 | 1 | |a Szleifer, I. | |
| 773 | 0 | |d American Chemical Society, 2015 |g v. 6 |h pp. 3534-3539 |k n. 18 |p J. Phys. Chem. Lett. |x 19487185 |w (AR-BaUEN)CENRE-4167 |t Journal of Physical Chemistry Letters | |
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| 856 | 4 | 0 | |u https://doi.org/10.1021/acs.jpclett.5b01315 |y DOI |
| 856 | 4 | 0 | |u https://hdl.handle.net/20.500.12110/paper_19487185_v6_n18_p3534_Tagliazucchi |y Handle |
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