Syntheses of 21-hydroxy-11,19-oxidopregn-4-ene-3,20-dione and 21-hydroxy-6,19-oxidopregn-4-ene-3,20-dione

The 21-hydroxy analogues of 11,19-oxidoprogesterone and 6,19-oxidoprogesterone have been synthesized from readily available materials. Hydroxylation at C-21 was effected with iodosobenzene (from phenyliodosodiacetate and methanolic potassium hydroxide) on a 20-ketopregnane. For the 11,19-oxido deriv...

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Detalles Bibliográficos
Autor principal: Veleiro, A.S
Otros Autores: Nevado, M.V, Monteserín, M.C, Burton, G.
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 1995
Acceso en línea:Registro en Scopus
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Registro en la Biblioteca Digital
Aporte de:Registro referencial: Solicitar el recurso aquí
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024 7 |2 scopus  |a 2-s2.0-0028985839 
024 7 |2 cas  |a aldosterone, 52-39-1, 6251-69-0; progesterone, 57-83-0; deoxycorticosterone, 64-85-7; 21-hydroxy-11,19-oxidopregn-4-ene-3,20-dione; 21-hydroxy-6,19-oxidopregn-4-ene-3,20-dione; Aldosterone, 52-39-1; Progesterone, 57-83-0 
040 |a Scopus  |b spa  |c AR-BaUEN  |d AR-BaUEN 
030 |a STEDA 
100 1 |a Veleiro, A.S. 
245 1 0 |a Syntheses of 21-hydroxy-11,19-oxidopregn-4-ene-3,20-dione and 21-hydroxy-6,19-oxidopregn-4-ene-3,20-dione 
260 |c 1995 
270 1 0 |m Burton, G.; Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires, Argentina 
506 |2 openaire  |e Política editorial 
504 |a Kamata, Matsui, Haga, Nakamura, Odaguchi, Itoh, Shimizu, Katoh, Aldosterone antagonists. 2. Synthesis and biological activities of 11,12-dehydropregnane derivatives (1987) J Med Chem, 30, pp. 1647-1658 
504 |a Brachet-Cota, Burton, An improved preparation of 11,19-oxidopregn-4-ene-3,20-dione and 6,19-oxidopregn-4-ene-3,11,20-trione (1990) Z Naturforsch [B], 45 b, pp. 711-715 
504 |a Galigniana, Vicent, Lantos, Burton, Ligand properties of 11,19-oxidoprogesterone (1993) A preliminary report, 81, pp. 333-340. , An Asoc Quim Argent 
504 |a Kirk, Yeoh, New syntheses of 1921-dihydroxy-4-ene-320-dione 21-hydroxy-19-norpregn-4-ene-320-dione and 11β1921-trihydroxypregn-4-ene-320-dione (1983) Journal of the Chemical Society, Perkin Transactions 1, pp. 2945-2950 
504 |a Deghenghi, The synthesis of 19-oxygenated cardenolides. I. A convenient preparation of 19-hydroxydesoxycorticosterone (1966) J Org Chem, 31, pp. 2427-2429 
504 |a Moriarty, John, Du, Hypervalent iodine in organic synthesis (1981) A novel route to the dihydroxyacetone side chain in pregnene series, pp. 641-642. , J Chem Soc Chem Commun 
504 |a Zemlicka, Beranek, Smrt, Preparation and methanolysis of uridine 6-azauridine and 6-azacytidine o-formyl derivatives (1962) Collection of Czechoslovak Chemical Communications, 27, pp. 2784-2795 
504 |a Moriarty, Hu, Gupta, Direct α-hydroxylation of ketones using iodosobenzene (1981) Tetrahedron Letters, 22, pp. 1283-1286 
504 |a Ringold, Stork, Steroids. XCIII. Introduction of the cortical hormone side-chain (1958) J Am Chem Soc, 80, p. 250 
520 3 |a The 21-hydroxy analogues of 11,19-oxidoprogesterone and 6,19-oxidoprogesterone have been synthesized from readily available materials. Hydroxylation at C-21 was effected with iodosobenzene (from phenyliodosodiacetate and methanolic potassium hydroxide) on a 20-ketopregnane. For the 11,19-oxido derivative, the hydroxylation was carried out on a precursor containing the oxido-bridge. This approach was not adequate for the 6,19-oxido steroid due to the very low yields encountered; hence in the latter case the order of introduction of the C-21 functionality and the oxido-bridge was reversed. © 1995.  |l eng 
536 |a Detalles de la financiación: Universidad de Buenos Aires 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas 
536 |a Detalles de la financiación: We thank Universidad de Buenos Aires, and CONICET (Argentina) for financial support of this work. 
593 |a Departamento de Química Orgánica, Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires, Argentina 
690 1 0 |a 21-HYDROXYLATION 
690 1 0 |a OXIDO-BRIDGED PREGNANES 
690 1 0 |a 21 HYDROXY 11,19 OXIDOPREGN 4 ENE 3,20 DIONE 
690 1 0 |a 21 HYDROXY 6,19 OXIDOPREGN 4 ENE 3,20 DIONE 
690 1 0 |a 21-HYDROXY-11,19-OXIDOPREGN-4-ENE-3,20-DIONE 
690 1 0 |a 21-HYDROXY-6,19-OXIDOPREGN-4-ENE-3,20-DIONE 
690 1 0 |a ALDOSTERONE 
690 1 0 |a DRUG DERIVATIVE 
690 1 0 |a PROGESTERONE 
690 1 0 |a 21 HYDROXY 11,19 OXIDOPREGN 4 ENE 3,20 DIONE 
690 1 0 |a 21 HYDROXY 6,19 OXIDOPREGN 4 ENE 3,20 DIONE 
690 1 0 |a DEOXYCORTICOSTERONE 
690 1 0 |a MINERALOCORTICOID RECEPTOR 
690 1 0 |a UNCLASSIFIED DRUG 
690 1 0 |a ACETYLATION 
690 1 0 |a ARTICLE 
690 1 0 |a CHEMICAL STRUCTURE 
690 1 0 |a CHEMISTRY 
690 1 0 |a HYDROXYLATION 
690 1 0 |a OXIDATION REDUCTION REACTION 
690 1 0 |a SYNTHESIS 
690 1 0 |a DRUG STRUCTURE 
690 1 0 |a DRUG SYNTHESIS 
690 1 0 |a STEROIDOGENESIS 
690 1 0 |a ACETYLATION 
690 1 0 |a ALDOSTERONE 
690 1 0 |a HYDROXYLATION 
690 1 0 |a MOLECULAR STRUCTURE 
690 1 0 |a OXIDATION-REDUCTION 
690 1 0 |a PROGESTERONE 
690 1 0 |a SUPPORT, NON-U.S. GOV'T 
700 1 |a Nevado, M.V. 
700 1 |a Monteserín, M.C. 
700 1 |a Burton, G. 
773 0 |d 1995  |g v. 60  |h pp. 268-271  |k n. 3  |p Steroids  |x 0039128X  |w (AR-BaUEN)CENRE-577  |t Steroids 
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856 4 0 |u https://hdl.handle.net/20.500.12110/paper_0039128X_v60_n3_p268_Veleiro  |y Handle 
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