Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties

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Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale,...

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Autor principal: Soler-Illia, G.J.A.A
Otros Autores: Angelomé, P.C, Fuertes, María Cecilia, Calvo, A., Wolosiuk, A., Zelcer, A., Bellino, M.G, Martínez, E.D
Formato: Capítulo de libro
Lenguaje:Inglés
Publicado: 2011
Acceso en línea:Registro en Scopus
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Biblioteca Central Dr. Luis F. Leloir (FCEN) de Universidad de Buenos Aires
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100 1 |a Soler-Illia, G.J.A.A. 
245 1 0 |a Mesoporous hybrid and nanocomposite thin films. A sol-gel toolbox to create nanoconfined systems with localized chemical properties 
260 |c 2011 
270 1 0 |m Soler-Illia, G. J. A. A.; Gerencia de Química, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. Gral Paz 1499 (B1650KNA), San Martín, Buenos Aires, Argentina; email: gsoler@cnea.gov.ar 
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506 |2 openaire  |e Política editorial 
520 3 |a Mesoporous Thin Films (MTF) can be created by combining sol-gel synthesis, template self-assembly and chemical surface modification. A wide palette of inorganic (oxides, phosphates, carbon-based, etc.) and hybrid organic-inorganic frameworks with a variety of composition, pore sizes, and nanoscale, organic or biological functions located in the inorganic skeleton, pore surface or pore interior can be obtained. The properties of the functional pore systems are tuned by the pore size and geometry, wall composition and surface features. These MTF with interesting electronic and optical controlled features are indeed a "nanofacility". Well-defined monodisperse sized pores also act as nanoreactors, or nanocavities with controlled environment and behaviour. In the last years, the production of accessible MTF, in which either the pore surface or pore volume can be modified by organic functional groups or nanoparticles has been thoroughly explored. Each highly controlled MTF originated from a reproducible and modular synthesis is in itself a building block for more complex structures, presenting order at different length scales (molecular, mesoscopic, macroscopic), and novel properties derived thereof. Selected examples of optical and chemical behaviour of these multiscale materials are presented to illustrate these points. © 2010 Springer Science+Business Media, LLC.  |l eng 
536 |a Detalles de la financiación: Maine Cancer Foundation 
536 |a Detalles de la financiación: Agencia Nacional de Promoción Científica y Tecnológica, PME 00038, PAE 2004 22711, PICT 34518, PICT 06-12057 
536 |a Detalles de la financiación: Consejo Nacional de Investigaciones Científicas y Técnicas, PIP 5191 
536 |a Detalles de la financiación: Acknowledgments Authors thank ABTLUS for partially funding access to the LNLS synchrotron facility, D02A-SAXS2 projects #4286/05, 4643/05, 4785/05, and D10A-XRD2 # 5872/06 project. Work partially funded by CONICET (PIP 5191, fellowship for MCF), ANPCyT (Grants PICT 06-12057, PICT 34518, PAE 2004 22711, PME 00038), and Gabbos. PCA, MCF, AZ and MGB thank CONI-CET for student and postdoctoral fellowships. PCA thanks CNEA for a graduate fellowship. EDM thanks Universidad de San Martín (UNSAM) for a graduate fellowship. GJAASI and AW are CONICET researchers. Authors thank Dr. M.C. Marchi for help in microscopy measurements, Prof. I. Torriani and Dr. T. Plivelic for assistance in SAXS, Dr. G. Kellermann for his help in XRR, Dr. L-Pietrasanta and S. Ludueña for the AFM image and P. Y. Steinberg for her help on methylene blue adsorption measurements. 
593 |a Gerencia de Química, Centro Atómico Constituyentes, Comisión Nacional de Energía Atómica, Av. Gral Paz 1499 (B1650KNA), San Martín, Buenos Aires, Argentina 
593 |a Departamento de Química Inorgánica, Analítica y Química Física, Facultad de Ciencias Exactas y Naturales, Ciudad Universitaria, Pabellón II, C1428EHA, Buenos Aires, Argentina 
690 1 0 |a FUNCTIONAL MATERIALS 
690 1 0 |a MESOPOROUS FILMS 
690 1 0 |a MESOPOROUS HYBRIDS 
690 1 0 |a NANOCHEMISTRY 
690 1 0 |a THIN FILMS 
690 1 0 |a BIOLOGICAL FUNCTIONS 
690 1 0 |a BUILDING BLOCKES 
690 1 0 |a CARBON-BASED 
690 1 0 |a CHEMICAL SURFACE MODIFICATION 
690 1 0 |a COMPLEX STRUCTURE 
690 1 0 |a CONTROLLED ENVIRONMENT 
690 1 0 |a DIFFERENT LENGTH SCALE 
690 1 0 |a MESOPOROUS FILMS 
690 1 0 |a MESOPOROUS HYBRIDS 
690 1 0 |a MESOPOROUS THIN FILMS 
690 1 0 |a MESOSCOPICS 
690 1 0 |a MODULAR SYNTHESIS 
690 1 0 |a MONODISPERSE 
690 1 0 |a MULTISCALES 
690 1 0 |a NANO CHEMISTRY 
690 1 0 |a NANO SCALE 
690 1 0 |a NANO-CAVITIES 
690 1 0 |a NANO-CONFINED SYSTEMS 
690 1 0 |a NANOCOMPOSITE THIN FILMS 
690 1 0 |a ORGANIC FUNCTIONAL GROUPS 
690 1 0 |a ORGANIC-INORGANIC 
690 1 0 |a PORE SURFACE 
690 1 0 |a PORE SYSTEM 
690 1 0 |a PORE VOLUME 
690 1 0 |a SELECTED EXAMPLES 
690 1 0 |a SOL-GEL SYNTHESIS 
690 1 0 |a SURFACE FEATURE 
690 1 0 |a CHEMICAL MODIFICATION 
690 1 0 |a CHEMICAL PROPERTIES 
690 1 0 |a FUNCTIONAL GROUPS 
690 1 0 |a FUNCTIONAL MATERIALS 
690 1 0 |a GELS 
690 1 0 |a NANOCOMPOSITE FILMS 
690 1 0 |a NANOCOMPOSITES 
690 1 0 |a OPTICAL TRANSFER FUNCTION 
690 1 0 |a PORE SIZE 
690 1 0 |a SOL-GEL PROCESS 
690 1 0 |a SOL-GELS 
690 1 0 |a SOLS 
690 1 0 |a SURFACES 
690 1 0 |a THIN FILMS 
690 1 0 |a MESOPOROUS MATERIALS 
700 1 |a Angelomé, P.C. 
700 1 |a Fuertes, María Cecilia 
700 1 |a Calvo, A. 
700 1 |a Wolosiuk, A. 
700 1 |a Zelcer, A. 
700 1 |a Bellino, M.G. 
700 1 |a Martínez, E.D. 
773 0 |d 2011  |g v. 57  |h pp. 299-312  |k n. 3  |p J Sol Gel Sci Technol  |x 09280707  |t Journal of Sol-Gel Science and Technology 
856 4 1 |u https://www.scopus.com/inward/record.uri?eid=2-s2.0-79954440541&doi=10.1007%2fs10971-010-2172-2&partnerID=40&md5=4655f8cdb4991fed3f1c5d1e09ab3ea3  |y Registro en Scopus 
856 4 0 |u https://doi.org/10.1007/s10971-010-2172-2  |y DOI 
856 4 0 |u https://hdl.handle.net/20.500.12110/paper_09280707_v57_n3_p299_SolerIllia  |y Handle 
856 4 0 |u https://bibliotecadigital.exactas.uba.ar/collection/paper/document/paper_09280707_v57_n3_p299_SolerIllia  |y Registro en la Biblioteca Digital 
961 |a paper_09280707_v57_n3_p299_SolerIllia  |b paper  |c PE 
962 |a info:eu-repo/semantics/article  |a info:ar-repo/semantics/artículo  |b info:eu-repo/semantics/publishedVersion 
999 |c 71739 

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