Phaseocyclopentenones A and B, Phytotoxic Penta - and Tetrasubstituted Cyclopentenones produced by Macrophomina phaseolina, the causal agent of Charcoal rot of Soybean in Argentina

Two new penta- and tetrasubstituted cyclopentenones, named phaseocyclopentenones A and B (1 and 2), together with guignardone A (3), were isolated from Macrophomina phaseolina cultures. The phytopathogenic fungus was isolated from infected soybean tissues showing charcoal rot symptoms in Argentina....

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Otros Autores: Masi, Marco, Sautua, Francisco José, Zatout, Roukia, Castaldi, Stefany, Arrico, Lorenzo, Isticato, Rachele, Pescitelli, Gennaro, Carmona, Marcelo Aníbal, Evidente, Antonio
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Acceso en línea:http://ri.agro.uba.ar/files/intranet/articulo/2021masi.pdf
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245 1 |a Phaseocyclopentenones A and B, Phytotoxic Penta - and Tetrasubstituted Cyclopentenones produced by Macrophomina phaseolina, the causal agent of Charcoal rot of Soybean in Argentina 
520 |a Two new penta- and tetrasubstituted cyclopentenones, named phaseocyclopentenones A and B (1 and 2), together with guignardone A (3), were isolated from Macrophomina phaseolina cultures. The phytopathogenic fungus was isolated from infected soybean tissues showing charcoal rot symptoms in Argentina. Charcoal rot is a devastating disease considering that soybean is one of the main legumes cultivated in the world. Phaseocyclopentenones A and B were characterized by 1D and 2D 1 H and 13C NMR spectroscopic and HRESIMS spectrometric data and chemical methods as 4-benzoyl-3,4,5-trihydroxy-2-phenylcyclopent-2- enone and 3,5-dihydroxy-2,4-diphenylcyclopent-2-enone, respectively. The relative configuration of phaseocyclopentenones A and B was assigned by 1 H and NOESY NMR methods, while their absolute configurations were assigned by electronic circular dichroism methods. When assayed on a nonhost plant (Solanum lycopersicum L.) by the leaf puncture assay, Phaseocyclopentenones A and B and guignardone A showed phytotoxic activity, while only 1 and 2 were toxic when tested on cuttings of the same plant. No phytotoxicity or antifungal activity was detected for the three compounds on the host plant soybean (Glycine max L.) and against some of its fungal pathogens, namely, Cercospora nicotianae and Colletotrichum truncatum, also isolated from infected soybean plants in Argentina. 
650 |2 Agrovoc  |9 26 
653 |a ASSYS 
653 |a METABOLISM 
653 |a PHENYLS 
653 |a PLANT DERIVED FOOD 
653 |a PLANTS 
700 1 |a Masi, Marco  |u Università di Napoli Federico II. Complesso Universitario Monte S. Angelo. Dipartimento di Scienze Chimiche. Napoli, Italy.  |9 73809 
700 1 |a Sautua, Francisco José  |u Universidad de Buenos Aires. Facultad de Agronomía. Departamento de Producción Vegetal. Cátedra de Fitopatología. Buenos Aires, Argentina.  |9 22833 
700 1 |a Zatout, Roukia  |u Università di Napoli Federico II. Complesso Universitario Monte S. Angelo. Dipartimento di Scienze Chimiche. Napoli, Italy.  |u Université des Frères Mentouri. Département de Biologie Appliquée. Laboratoire de Mycologie, de Biotechnologie et de l’Activité Microbienne (LaMyBAM). Constantine, Algeria.  |9 73810 
700 1 |a Castaldi, Stefany  |u Università di Napoli Federico II. Complesso Universitario Monte S. Angelo. Dipartimento di Biologia, Napoli, Italy.  |9 73811 
700 1 |a Arrico, Lorenzo  |u Università di Pisa. Dipartimento di Chimica e Chimica Industriale. Pisa, Italy.  |9 73812 
700 1 |a Isticato, Rachele  |u Università di Napoli Federico II. Dipartimento di Biologia. Complesso Universitario Monte S. Angelo, Napoli, Italy.  |9 73813 
700 1 |a Pescitelli, Gennaro  |u Università di Pisa. Dipartimento di Chimica e Chimica Industriale. Pisa, Italy.  |9 73814 
700 1 |a Carmona, Marcelo Aníbal  |u Universidad de Buenos Aires. Facultad de Agronomía. Departamento de Producción Vegetal. Cátedra de Fitopatología. Buenos Aires, Argentina.  |9 3109 
700 1 |a Evidente, Antonio  |u Università di Napoli Federico II. Complesso Universitario Monte S. Angelo. Dipartimento di Scienze Chimiche. Napoli, Italy.  |9 73877 
773 0 |t Journal of natural products  |w SECS000707  |g Vol.84, no.2 (2021), p.459-465, grafs., tbls., fot. 
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