The potentiodynamic behaviour of iridium electrodes in NaHSO<sub>4</sub> - KHSO<sub>4</sub> melts

Noble metal electrodes in aqueous solutions under a triangular potential sweep display current peaks due to the electrosorption and electrodesorption of hydrogen and oxygen species [1-7]. In molten bisulphate electrolytes these characteristics were previously observed for platinum [8-11] and are als...

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Detalles Bibliográficos
Autores principales: Zerbino, Jorge Omar, Tacconi, Norma R. de, Calandra, Alfredo J., Arvia, Alejandro Jorge
Formato: Articulo Comunicacion
Lenguaje:Español
Publicado: 1977
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Acceso en línea:http://sedici.unlp.edu.ar/handle/10915/118262
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Sumario:Noble metal electrodes in aqueous solutions under a triangular potential sweep display current peaks due to the electrosorption and electrodesorption of hydrogen and oxygen species [1-7]. In molten bisulphate electrolytes these characteristics were previously observed for platinum [8-11] and are also common for iridium. The electrochemical behaviour of iridium (1 mm diameter wire, Johnson Matthey, 1.0 cm<sup>2</sup> apparent area) was studied in the NaHSO<sub>4</sub>-KHSO<sub>4</sub> melts at 180-300°C using a conventional three compartment electrolysis cell. Its potential was referred to a Pt/H<sub>2</sub>(1 atm)/KHSO<sub>4</sub>(melt) electrode.