Convenient synthesis of the immunogenic glycolipid BbGL1

A simple and efficient method to synthesize the immunogenic glycolipid BbGL1 is introduced. Two simple steps were required to obtain the desired product in good yield. First, a highly efficient glycosylation of cholesterol using galactosyl trichloroacetimidate as a donor was performed to produce cho...

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Autores principales: Jäger, Sebastián N., Porta, Exequiel Oscar Jesús, Labadie, Guillermo Roberto
Formato: article artículo acceptedVersion
Lenguaje:Inglés
Publicado: Elsevier 2020
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Acceso en línea:http://hdl.handle.net/2133/18280
http://hdl.handle.net/2133/18280
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Sumario:A simple and efficient method to synthesize the immunogenic glycolipid BbGL1 is introduced. Two simple steps were required to obtain the desired product in good yield. First, a highly efficient glycosylation of cholesterol using galactosyl trichloroacetimidate as a donor was performed to produce cholesteryl-β-d-galactoside. Finally, an efficient palmitoylation on the C6–OH of the galactose of the synthesized saponin using sym-collidine and acyl chloride under microwave heating that produced BbGL1 in good yield. The procedure is a convenient and cheaper alternative to the reported procedures allowing a rapid preparation of multiple analogs and conjugates.